J06:0010a	-	YB	<majbrk>	-	[Oh.Oh]
J06:0010b	-	AT	The	the	[O[S[Ns:s.
J06:0010c	-	JJ	thermal	thermal	.
J06:0010d	-	NN1n	exchange	exchange	.
J06:0010e	-	IO	of	of	[Po.
J06:0010f	-	NN1u	chlorine	chlorine	.Po]
J06:0010g	-	II	between	between	[P.
J06:0010h	-	FO	<formul>	-	[N.
J06:0010i	-	CC	and	and	[N+.
J06:0010j	-	JJ	liquid	liquid	.
J06:0010k	-	FO	<formul>	-	.N+]N]P]Ns:s]
J06:0010m	-	VBZ	is	be	[Vzb.Vzb]
J06:0020a	-	RR	readily	readily	[R:h.R:h]
J06:0020b	-	JJ	measurable	measurable	[J:e.J:e]
J06:0020c	-	II	at	at	[P:p.
J06:0020d	-	NN2	temperatures	temperature	[Np.
J06:0020e	-	II	in	in	[P.
J06:0020f	-	AT	the	the	[Ns.
J06:0020g	-	NN1c	range	range	.
J06:0020h	-	IO	of	of	[Po.
J06:0020i	-	MCn	180	-	[Nu.
J06:0020j	-	NNU	+<deg>	-	.
J06:0020k	-	CC	and	and	[R+.
J06:0020m	-	RL	above	above	.R+]Nu]Po]Ns]P]Np]P:p]S]
J06:0020n	-	YF	+.	-	.
J06:0020p	-	AT	The	the	[S[Ns:s101.
J06:0030a	-	JJ	photochemical	photochemical	.
J06:0030b	-	NN1n	exchange	exchange	.Ns:s101]
J06:0030c	-	VVZi	occurs	occur	[Vz.Vz]
J06:0030d	-	IW	with	with	[P:b.
J06:0030e	-	AT1	a	a	[Ns.
J06:0030f	-	NN1c	quantum	quantum	.
J06:0030g	-	NN1n	yield	yield	.
J06:0030h	-	IO	of	of	[Po.
J06:0030i	-	AT	the	the	[Ns.
J06:0030j	-	NN1n	order	order	.
J06:0030k	-	IO	of	of	[Po.
J06:0040a	-	NN1n	unity	unity	.Po]Ns]Po]Ns]P:b]
J06:0040b	-	II	in	in	[P:p.
J06:0040c	-	AT	the	the	[Ns.
J06:0040d	-	JJ	liquid	liquid	.
J06:0040e	-	NN1c	phase	phase	.Ns]P:p]
J06:0040f	-	II	at	at	[P:p.
J06:0040g	-	MCn	65	-	[Nu.
J06:0040h	-	NNU	+<deg>	-	.Nu]P:p]
J06:0040i	-	YG	-	-	[Tg:h[s101.s101]
J06:0040j	-	VVGt	using	use	[Vg.Vg]
J06:0040k	-	NN1n	light	light	[Ns:o103.
J06:0040m	-	YG	-	-	[Tn[S103.S103]
J06:0040n	-	VVNt	absorbed	absorb	[Vn.Vn]
J06:0040p	-	RRx	only	only	[R:m.R:m]
J06:0040q	-	IIb	by	by	[Pb:a.
J06:0040r	-	AT	the	the	[N.
J06:0040s	-	FO	<formul>	-	.N]Pb:a]Tn]Ns:o103]Tg:h]S]
J06:0040t	-	YF	+.	-	.
J06:0050a	-	II	In	in	[S[P:p.
J06:0050b	-	AT	the	the	[Ns.
J06:0050c	-	NN1n	gas	gas	.
J06:0050d	-	NN1c	phase	phase	.Ns]P:p]
J06:0050e	-	YC	+,	-	.
J06:0050f	-	IW	with	with	[P:b.
J06:0050g	-	FO	<formul>	-	[N.
J06:0050h	-	IO	of	of	[Po.
J06:0050i	-	FO	<formul>	-	.Po]
J06:0050j	-	CC	and	and	[N+.
J06:0050k	-	FO	<formul>	-	.
J06:0050m	-	IO	of	of	[Po.
J06:0050n	-	FO	<formul>	-	.Po]N+]N]P:b]
J06:0050p	-	YC	+,	-	.
J06:0050q	-	NN1c	quantum	quantum	[Np:S.
J06:0050r	-	NN2	yields	yield	.
J06:0051a	-	IO	of	of	[Po.
J06:0051b	-	AT	the	the	[Ns.
J06:0060a	-	NN1n	order	order	.
J06:0060b	-	IO	of	of	[Po.
J06:0060c	-	FO	<formul>	-	.Po]Ns]Po]Np:S]
J06:0060d	-	VH0	have	have	[Vfp.
J06:0060e	-	VBN	been	be	.
J06:0060f	-	VVNv	observed	observe	.Vfp]
J06:0060g	-	II	at	at	[P:p.
J06:0060h	-	MCn	85	-	[Nu.
J06:0060i	-	NNU	+<deg>	-	.Nu]P:p]S]
J06:0060j	-	YF	+.	-	.
J06:0060k	-	II	Despite	despite	[S[P:c.
J06:0060m	-	JJ	extensive	extensive	[Np.
J06:0060n	-	NN2	attempts	attempt	.
J06:0070a	-	TO	to	to	[Ti[Vi.
J06:0070b	-	VV0v	obtain	obtain	.Vi]
J06:0070c	-	RR	highly	highly	[Np:o[J.
J06:0070d	-	JJ	pure	pure	.J]
J06:0070e	-	NN2	reagents	reagent	.Np:o]Ti]Np]P:c]
J06:0070f	-	YC	+,	-	.
J06:0070g	-	JJ	serious	serious	[Ns:S.
J06:0070h	-	NN1n	difficulty	difficulty	.Ns:S]
J06:0070i	-	VBDZ	was	be	[Vsp.
J06:0070j	-	VVNt	experienced	experience	.Vsp]
J06:0070k	-	II	in	in	[P:r.
J06:0080a	-	VVGv	obtaining	obtain	[Tg[Vg.Vg]
J06:0080b	-	JJ	reproducible	reproducible	[Np:o.
J06:0080c	-	NN2	rates	rate	.
J06:0080d	-	IO	of	of	[Po.
J06:0080e	-	NN1n	reaction	reaction	.Po]Np:o]Tg]P:r]S]
J06:0080f	-	YF	+.	-	.
J06:0080g	-	PPH1	It	it	[S[Ni:S.Ni:S]
J06:0080h	-	VVZi	appears	appear	[Vz.Vz]
J06:0080i	-	JJ	possible	possible	[J:e.J:e]
J06:0080j	-	TO	to	to	[Ti:s[Vi.
J06:0080k	-	VV0v	set	set	.Vi]
J06:0090a	-	AT1	a	a	[Ns:o.
J06:0090b	-	JJR	lower	low	.
J06:0090c	-	NN1c	limit	limit	.
J06:0090d	-	IO	of	of	[Po.
J06:0090e	-	RGi	about	about	[N.
J06:0090f	-	FO	<formul>	-	.N]Po]Ns:o]
J06:0090g	-	IF	for	for	[Tf:r.
J06:0090h	-	AT	the	the	[Ns:s.
J06:0090i	-	NN1c	activation	activation	.
J06:0090j	-	NN1n	energy	energy	.
J06:0090k	-	IO	of	of	[Po.
J06:0090m	-	AT	the	the	[Ns.
J06:0090n	-	NN1n	abstraction	abstraction	.
J06:0100a	-	IO	of	of	[Po.
J06:0100b	-	AT1	a	a	[Ns.
J06:0100c	-	NN1u	chlorine	chlorine	.
J06:0100d	-	NN1c	atom	atom	.Ns]Po]
J06:0100e	-	II	from	from	[P.
J06:0100f	-	AT1	a	a	[Ns.
J06:0100g	-	NN1n	carbon	carbon	[Ns.
J06:0100h	-	NN1n	tetrachloride	tetrachloride	.Ns]
J06:0100i	-	NN1c	molecule	molecule	.Ns]P]
J06:0100j	-	IIb	by	by	[Pb.
J06:0100k	-	AT1	a	a	[Ns.
J06:0100m	-	NN1u	chlorine	chlorine	.
J06:0110a	-	NN1c	atom	atom	.Ns]Pb]Ns]Po]Ns:s]
J06:0110b	-	TO	to	to	[Vi.
J06:0110c	-	VV0v	form	form	.Vi]
J06:0110d	-	FO	<formul>	-	[Nj:o.
J06:0110e	-	JJ	radical	radical	.Nj:o]Tf:r]Ti:s]S]
J06:0110f	-	YF	+.	-	.
J06:0110g	-	AT	The	the	[S[Ns:S105.
J06:0110h	-	NN1c	rate	rate	.
J06:0110i	-	IO	of	of	[Po.
J06:0110j	-	AT	the	the	[Ns.
J06:0110k	-	NN1n	gas	gas	[Ns.
J06:0110m	-	NN1c	phase	phase	.Ns]
J06:0110n	-	NN1n	exchange	exchange	.
J06:0110p	-	NN1n	reaction	reaction	.Ns]Po]Ns:S105]
J06:0120a	-	VVZi	appears	appear	[Vz.Vz]
J06:0120b	-	YG	-	-	[Ti:s[s105.s105]
J06:0120c	-	TO	to	to	[Vib.
J06:0120d	-	VB0	be	be	.Vib]
J06:0120e	-	JJ	proportional	proportional	[Jh:e.
J06:0120f	-	IIt	to	to	[P.
J06:0120g	-	AT	the	the	[Ns.
J06:0120h	-	MDo	first	first	.
J06:0120i	-	NN1n	power	power	.
J06:0120j	-	IO	of	of	[Po.
J06:0120k	-	AT	the	the	[Ns.
J06:0120m	-	VVNt	absorbed	absorb	[Ns[Tn[Vn.Vn]Tn]
J06:0120n	-	NN1n	light	light	.Ns]
J06:0130a	-	NN1n	intensity	intensity	.Ns]Po]Ns]P]Jh:e]Ti:s]
J06:0130b	-	VVGt	indicating	indicate	[Tg:b[Vg.Vg]
J06:0130c	-	CST	that	that	[Fn:o.
J06:0130d	-	AT	the	the	[Np:S.
J06:0130e	-	JJ	radical	radical	.
J06:0130f	-	NN2	intermediates	intermediate	.Np:S]
J06:0130g	-	VBR	are	be	[Vap.
J06:0130h	-	VVNv	removed	remove	.Vap]
J06:0130i	-	II	at	at	[P:p.
J06:0140a	-	AT	the	the	[Np.
J06:0140b	-	NN2	walls	wall	.Np]
J06:0140c	-	CCr	or	or	[Pb+.
J06:0140d	-	IIb	by	by	.
J06:0140e	-	NN1n	reaction	reaction	[Ns.
J06:0140f	-	IW	with	with	[P.
J06:0140g	-	AT1	an	an	[Ns.
J06:0140h	-	NN1n	impurity	impurity	.Ns]P]Ns]Pb+]P:p]
J06:0140i	-	RRR	rather	rather	[R:m.
J06:0140j	-	CSN	than	than	[Fc.
J06:0140k	-	IIb	by	by	[Pb:a.
J06:0140m	-	JJ	bimolecular	bimolecular	[Np[J.
J06:0150a	-	JJ	radical	radical	.J]
J06:0150b	-	NN1n	combination	combination	.
J06:0150c	-	NN2	reactions	reaction	.Np]Pb:a]Fc]R:m]Fn:o]Tg:b]S]
J06:0150d	-	YF	+.	-	.O]
J06:0150e	-	YBL	<bmajhd>	-	[Oh.
J06:0150f	-	NN1n	INTRODUCTION	introduction	.
J06:0150g	-	YBR	<emajhd>	-	.Oh]
J06:0150h	-	II21	Because	because	[O[S[P:c[II=.
J06:0150i	-	II22	of	of	.II=]
J06:0150j	-	AT	the	the	[Ns.
J06:0150k	-	NN1u	simplicity	simplicity	.
J06:0160a	-	IO	of	of	[Po.
J06:0160b	-	AT	the	the	[Np.
J06:0160c	-	NN2	molecules	molecule	.Np]Po]Ns]P:c]
J06:0160d	-	YC	+,	-	.
J06:0160e	-	JJ	isotopic	isotopic	[Np:S107.
J06:0160f	-	NN1n	exchange	exchange	.
J06:0160g	-	NN2	reactions	reaction	.
J06:0160h	-	II	between	between	[P.
J06:0160i	-	JJ	elemental	elemental	[Np.
J06:0170a	-	NN2	halogens	halogen	.
J06:0170b	-	CC	and	and	[Np+.
J06:0170c	-	AT	the	the	.
J06:0170d	-	JJ	corresponding	corresponding	.
J06:0170e	-	NN1n	carbon	carbon	.
J06:0170f	-	NN2	tetrahalides	tetrahalide	.Np+]Np]P]Np:S107]
J06:0170g	-	VMd	would	will	[Vdc.
J06:0170h	-	VV0i	appear	appear	.Vdc]
J06:0170i	-	YG	-	-	[Ti:s[s107.s107]
J06:0170j	-	TO	to	to	[Vi.
J06:0170k	-	VV0v	offer	offer	.Vi]
J06:0180a	-	RR	particularly	particularly	[Np:o[J.
J06:0180b	-	JJ	fruitful	fruitful	.J]
J06:0180c	-	NN2	possibilities	possibility	.
J06:0180d	-	IF	for	for	[P.
J06:0180e	-	VVGv	obtaining	obtain	[Tg[Vg.Vg]
J06:0180f	-	JJ	unambiguous	unambiguous	[N:o.
J06:0180g	-	JJ	basic	basic	.
J06:0190a	-	JJ	kinetic	kinetic	.
J06:0190b	-	NNu	data	data	.N:o]Tg]P]Np:o]Ti:s]S]
J06:0190c	-	YF	+.	-	.
J06:0190d	-	PPH1	It	it	[S[Ni:S.Ni:S]
J06:0190e	-	VMd	would	will	[Vdc.
J06:0190f	-	VV0i	appear	appear	.Vdc]
J06:0190g	-	CST	that	that	[Fn:s.
J06:0190h	-	PPH1	it	it	[Ni:S.Ni:S]
J06:0190i	-	VMd	should	shall	[Vdcb.
J06:0190j	-	VB0	be	be	.Vdcb]
J06:0190k	-	JJ	possible	possible	[J:e.J:e]
J06:0190m	-	TO	to	to	[Ti:s[Vi.
J06:0190n	-	VV0v	determine	determine	.Vi]
J06:0200a	-	JJ	unique	unique	[Np:o.
J06:0200b	-	NN2	mechanisms	mechanism	.
J06:0200c	-	IF	for	for	[P.
J06:0200d	-	AT	the	the	[Np.
J06:0200e	-	JJ	thermal	thermal	[JJ&.
J06:0200f	-	CC	and	and	[JJ+.
J06:0200g	-	JJ	photochemical	photochemical	.JJ+]JJ&]
J06:0200h	-	NN2	reactions	reaction	.
J06:0200i	-	II	in	in	[P.
J06:0200j	-	LE	both	both	[Np.
J06:0210a	-	AT	the	the	.
J06:0210b	-	JJ	liquid	liquid	[JJ&.
J06:0210c	-	CC	and	and	[NN1n+.
J06:0210d	-	NN1n	gas	gas	.NN1n+]JJ&]
J06:0210e	-	NN2	phases	phase	.Np]P]Np]P]Np:o]
J06:0210f	-	CC	and	and	[Ti+.
J06:0210g	-	TO	to	to	[Vi.
J06:0210h	-	VV0v	determine	determine	.Vi]
J06:0210i	-	NN2	values	value	[N:o.
J06:0210j	-	IF	for	for	[P.
J06:0210k	-	NN1c	activation	activation	[Np.
J06:0210m	-	NN2	energies	energy	.
J06:0220a	-	IO	of	of	[Po.
J06:0220b	-	DDi	some	some	[Dp.
J06:0220c	-	IO	of	of	[Po.
J06:0220d	-	AT	the	the	[Np.
J06:0220e	-	JJ	intermediate	intermediate	.
J06:0220f	-	NN2	reactions	reaction	.
J06:0220g	-	IO	of	of	[Po.
J06:0220h	-	NN2	atoms	atom	[Np.
J06:0220i	-	CC	and	and	[Np+.
J06:0220j	-	JJ	free	free	.
J06:0220k	-	NN2	radicals	radical	.Np+]Np]Po]Np]Po]Dp]Po]Np]P]
J06:0220m	-	YC	+,	-	.
J06:0230a	-	CC31	as	as	[Ns+[CC=.
J06:0230b	-	CC32	well	well	.
J06:0230c	-	CC33	as	as	.CC=]
J06:0230d	-	NN1u	information	information	.
J06:0230e	-	II	on	on	[P.
J06:0230f	-	AT	the	the	[Ns.
J06:0230g	-	NN1n	heat	heat	.
J06:0230h	-	IO	of	of	[Po.
J06:0230i	-	NN1u	dissociation	dissociation	.Po]
J06:0230j	-	IO	of	of	[Po.
J06:0230k	-	AT	the	the	[Ns.
J06:0230m	-	NN1n	carbon	carbon	[N.
J06:0230n	-	YH	+<hyphen>	-	.
J06:0230p	-	NN1n	+halogen	halogen	.N]
J06:0240a	-	NN1c	bond	bond	.Ns]Po]Ns]P]Ns+]N:o]Ti+]Ti:s]Fn:s]S]
J06:0240b	-	YF	+.	-	.
J06:0240c	-	AT	The	the	[S[Ns:s.
J06:0240d	-	NN1n	reaction	reaction	.
J06:0240e	-	IO	of	of	[Po.
J06:0240f	-	NN1u	chlorine	chlorine	.Po]
J06:0240g	-	IW	with	with	[P.
J06:0240h	-	NN1n	carbon	carbon	[Ns.
J06:0240i	-	NN1u	tetrachloride	tetrachloride	.Ns]P]Ns:s]
J06:0240j	-	VVDi	seemed	seem	[Vd.Vd]
J06:0250a	-	RR	particularly	particularly	[Tn:e[R:h.R:h]
J06:0250b	-	VVNv	suited	suit	[Vn.Vn]
J06:0250c	-	IF	for	for	[P:u.
J06:0250d	-	DAz	such	such	[Np.
J06:0250e	-	NN2	studies	study	.Np]P:u]Tn:e]S]
J06:0250f	-	YF	+.	-	.
J06:0250g	-	PPH1	It	it	[S[Ni:S.Ni:S]
J06:0250h	-	VMd	should	shall	[Vdcb.
J06:0250i	-	VB0	be	be	.Vdcb]
J06:0250j	-	JJ	possible	possible	[J:e.J:e]
J06:0250k	-	TO	to	to	[Ti:s[Vi.
J06:0250m	-	VV0v	prepare	prepare	.Vi]
J06:0260a	-	RG	very	very	[Ns:o[J.
J06:0260b	-	JJ	pure	pure	.J]
J06:0260c	-	NN1u	chlorine	chlorine	.Ns:o]
J06:0260d	-	IIb	by	by	[Pb:h.
J06:0260e	-	NN1n	oxidation	oxidation	[Ns:109.
J06:0260f	-	IO	of	of	[Po.
J06:0260g	-	JJ	inorganic	inorganic	[Np.
J06:0260h	-	NN2	chlorides	chloride	.Np]Po]
J06:0260i	-	II	on	on	[P.
J06:0260j	-	AT1	a	a	[Ns.
J06:0260k	-	NN1c	vacuum	vacuum	.
J06:0270a	-	NN1n	system	system	.Ns]P]
J06:0270b	-	YG	-	-	[Tn[S109.S109]
J06:0270c	-	VVNv	followed	follow	[Vn.Vn]
J06:0270d	-	IIb	by	by	[Pb:a.
J06:0270e	-	JJ	multiple	multiple	[Ns.
J06:0270f	-	NN1n	distillation	distillation	.
J06:0270g	-	IO	of	of	[Po.
J06:0270h	-	AT	the	the	[Ns.
J06:0270i	-	NN1n	liquid	liquid	.Ns]Po]Ns]Pb:a]Tn]Ns:109]Pb:h]Ti:s]S]
J06:0270j	-	YF	+.	-	.
J06:0270k	-	PPH1	It	it	[S[Ni:S.Ni:S]
J06:0270m	-	VMd	should	shall	[Vdcb.
J06:0270n	-	VB0	be	be	.Vdcb]
J06:0280a	-	JJ	possible	possible	[J:e.J:e]
J06:0280b	-	TO	to	to	[Ti:s[Vi.
J06:0280c	-	VV0t	free	free	.Vi]
J06:0280d	-	NN1n	carbon	carbon	[Ns:o.
J06:0280e	-	NN1u	tetrachloride	tetrachloride	.Ns:o]
J06:0280f	-	IO	of	of	[Po:u.
J06:0280g	-	DDy	any	any	[Np.
J06:0280h	-	VVGi	interfering	interfere	[Tg[Vg.Vg]Tg]
J06:0280i	-	NN2	substances	substance	.Np]Po:u]
J06:0280j	-	IIb	by	by	[Pb:h.
J06:0290a	-	AT	the	the	[Np:111.
J06:0290b	-	JJ	usual	usual	.
J06:0290c	-	NN1n	purification	purification	.
J06:0290d	-	NN2	methods	method	.
J06:0290e	-	YG	-	-	[Tn[S111.S111]
J06:0290f	-	VVNv	followed	follow	[Vn.Vn]
J06:0290g	-	IIb	by	by	[Pb:a.
J06:0290h	-	NN1n	prechlorination	prechlorination	[Ns.
J06:0290i	-	II21	prior	prior	[P[II=.
J06:0290j	-	II22	to	to	.II=]
J06:0300a	-	NN1n	addition	addition	[Ns.
J06:0300b	-	IO	of	of	[Po.
J06:0300c	-	JJ	radioactive	radioactive	[Ns.
J06:0300d	-	NN1u	chlorine	chlorine	.Ns]Po]Ns]P]Ns]Pb:a]Tn]Np:111]Pb:h]Ti:s]S]
J06:0300e	-	YF	+.	-	.
J06:0300f	-	RR	Furthermore	furthermore	[S[R:m.R:m]
J06:0300g	-	YC	+,	-	.
J06:0300h	-	AT	the	the	[Ns:S.
J06:0300i	-	NN1n	exchange	exchange	.Ns:S]
J06:0300j	-	VMd	would	will	[Vdcep.
J06:0300k	-	XX	not	not	.
J06:0310a	-	VB0	be	be	.
J06:0310b	-	VVNt	expected	expect	.Vdcep]
J06:0310c	-	TO	to	to	[Ti:s[Vib.
J06:0310d	-	VB0	be	be	.Vib]
J06:0310e	-	JJ	sensitive	sensitive	[Jh:e.
J06:0310f	-	IIt	to	to	[P.
J06:0310g	-	NN1n	trace	trace	[Np.
J06:0310h	-	NN2	amounts	amount	.
J06:0310i	-	IO	of	of	[Po.
J06:0310j	-	NN2	impurities	impurity	.Po]Np]P]Jh:e]Ti:s]
J06:0310k	-	CS	because	because	[Fa:c.
J06:0310m	-	PPH1	it	it	[Ni:s.Ni:s]
J06:0320a	-	VMd	would	will	[Vdceb.
J06:0320b	-	XX	not	not	.
J06:0320c	-	VB0	be	be	.Vdceb]
J06:0320d	-	JJ	apt	apt	[Jh:e.
J06:0320e	-	TO	to	to	[Ti[Vib.
J06:0320f	-	VB0	be	be	.Vib]
J06:0320g	-	AT1	a	a	[Ns:e.
J06:0320h	-	NN1c	chain	chain	.
J06:0320i	-	NN1n	reaction	reaction	.Ns:e]Ti]Jh:e]
J06:0320j	-	ICSt	since	since	[Fa:c.
J06:0320k	-	AT	the	the	[Ns:S.
J06:0320m	-	NN1c	activation	activation	.
J06:0320n	-	NN1n	energy	energy	.
J06:0320p	-	IF	for	for	[P.
J06:0330a	-	NN1n	abstraction	abstraction	[Ns.
J06:0330b	-	IO	of	of	[Po.
J06:0330c	-	NN1u	chlorine	chlorine	.Po]
J06:0330d	-	IIb	by	by	[Pb.
J06:0330e	-	AT1	a	a	[Ns.
J06:0330f	-	NN1u	chlorine	chlorine	.
J06:0330g	-	NN1c	atom	atom	.Ns]Pb]Ns]P]Ns:S]
J06:0330h	-	VMd	would	will	[Vdcp.
J06:0330i	-	VB0	be	be	.
J06:0330j	-	VVNt	expected	expect	.Vdcp]
J06:0330k	-	TO	to	to	[Ti:s[Vib.
J06:0330m	-	VB0	be	be	.Vib]
J06:0340a	-	RGf	too	too	[J:e.
J06:0340b	-	JJ	high	high	.J:e]Ti:s]Fa:c]Fa:c]
J06:0340c	-	YS	+;	-	.
J06:0340d	-	RR	also	also	[S-[R:m.R:m]
J06:0340e	-	PPH1	it	it	[Ni:S.Ni:S]
J06:0340f	-	VMd	would	will	[Vdcp.
J06:0340g	-	VB0	be	be	.
J06:0340h	-	VVNt	expected	expect	.Vdcp]
J06:0340i	-	CST	that	that	[Fn:o.
J06:0340j	-	FO	<formul>	-	[N:s.N:s]
J06:0340k	-	VMd	would	will	[Vdc.
J06:0340m	-	VV0i	compete	compete	.Vdc]
J06:0340n	-	RG	very	very	[R:h.
J06:0340p	-	RR	effectively	effectively	.R:h]
J06:0350a	-	IW	with	with	[P:u.
J06:0350b	-	DDy	any	any	[Np.
J06:0350c	-	NN2	impurities	impurity	.Np]P:u]
J06:0350d	-	IIa	as	as	[P:e.
J06:0350e	-	AT1	a	a	[Ns.
J06:0350f	-	NN1c	scavenger	scavenger	.
J06:0350g	-	IF	for	for	[P.
J06:0350h	-	FO	<formul>	-	[Np.
J06:0350i	-	NN2	radicals	radical	.Np]P]Ns]P:e]Fn:o]S-]S]
J06:0350j	-	YF	+.	-	.
J06:0350k	-	II21	Contrary	contrary	[S[P:c[II=.
J06:0360a	-	II22	to	to	.II=]
J06:0360b	-	DD2i	these	these	[Np.
J06:0360c	-	NN2	expectations	expectation	.Np]P:c]
J06:0360d	-	PPIS2	we	we	[Nap:s.Nap:s]
J06:0360e	-	VH0	have	have	[Vf.
J06:0360f	-	VVNt	found	find	.Vf]
J06:0360g	-	PPH1	it	it	[Ni:O.Ni:O]
J06:0360h	-	JJ	impossible	impossible	[J:j.J:j]
J06:0360i	-	TO	to	to	[Ti:o[Vi.
J06:0360j	-	VV0v	obtain	obtain	.Vi]
J06:0360k	-	AT	the	the	[Nus:o113.
J06:0360m	-	NNU1n	degree	degree	.
J06:0370a	-	IO	of	of	[Po.
J06:0370b	-	NN1n	reproducibility	reproducibility	.Po]
J06:0370c	-	PN1o	one	one	[Fr[Ns:s.Ns:s]
J06:0370d	-	VMd	would	will	[Vdc.
J06:0370e	-	VV0v	wish	wish	.Vdc]
J06:0370f	-	YG	-	-	[o113.o113]Fr]Nus:o113]Ti:o]
J06:0370g	-	YC	+,	-	.
J06:0370h	-	RR	even	even	[P:h.
J06:0370i	-	IW	with	with	.
J06:0370j	-	JJ	extensive	extensive	[Np.
J06:0370k	-	NN2	efforts	effort	.
J06:0370m	-	TO	to	to	[Ti[Vi.
J06:0370n	-	VV0v	prepare	prepare	.Vi]
J06:0380a	-	RR	especially	especially	[Np:o[J.
J06:0380b	-	JJ	pure	pure	.J]
J06:0380c	-	NN2	reagents	reagent	.Np:o]Ti]Np]P:h]S]
J06:0380d	-	YF	+.	-	.
J06:0380e	-	PPIS2	We	we	[S[Nap:s.Nap:s]
J06:0380f	-	VBR	are	be	[Vau.
J06:0380g	-	VVGv	reporting	report	.Vau]
J06:0380h	-	DD2i	these	these	[Np:o.
J06:0380i	-	NN2	investigations	investigation	.Np:o]
J06:0390a	-	RLh	here	here	[Rw:p.Rw:p]
J06:0390b	-	RR	briefly	briefly	[R:h.R:h]
J06:0390c	-	II21	because	because	[P:c[II=.
J06:0390d	-	II22	of	of	.II=]
J06:0390e	-	APPGh2	their	their	[Ns.
J06:0390f	-	NN1u	relevancy	relevancy	.
J06:0390g	-	IIt	to	to	[P.
J06:0390h	-	NN2	problems	problem	[Np.
J06:0390i	-	IO	of	of	[Po.
J06:0390j	-	AT	the	the	[Ns.
J06:0390k	-	NN1n	study	study	.
J06:0390m	-	IO	of	of	[Po.
J06:0390n	-	RR	apparently	apparently	[Np[J.
J06:0400a	-	JJ	simple	simple	.J]
J06:0400b	-	NN1n	exchange	exchange	.
J06:0400c	-	NN2	reactions	reaction	.
J06:0400d	-	IO	of	of	[Po.
J06:0400e	-	NN1u	chlorine	chlorine	.Po]Np]Po]Ns]Po]Np]P]Ns]
J06:0400f	-	CC	and	and	[Fa+.
J06:0400g	-	CS	because	because	.
J06:0400h	-	AT	the	the	[Np:s.
J06:0400i	-	NN2	results	result	.Np:s]
J06:0410a	-	VV0t	furnish	furnish	[V.V]
J06:0410b	-	DDi	some	some	[Ns:o.
J06:0410c	-	NN1u	information	information	.
J06:0410d	-	II	on	on	[P.
J06:0410e	-	AT	the	the	[Ns.
J06:0410f	-	NN1c	activation	activation	.
J06:0410g	-	NN1n	energy	energy	.
J06:0410h	-	IF	for	for	[P.
J06:0410i	-	NN1n	abstraction	abstraction	[Ns.
J06:0410j	-	IO	of	of	[Po.
J06:0420a	-	NN1u	chlorine	chlorine	[Np.
J06:0420b	-	NN2	atoms	atom	.Np]Po]
J06:0420c	-	II	from	from	[P.
J06:0420d	-	NN1n	carbon	carbon	[Ns.
J06:0420e	-	NN1u	tetrachloride	tetrachloride	.Ns]P]Ns]P]Ns]P]Ns:o]Fa+]P:c]S]
J06:0420f	-	YF	+.	-	.O]
J06:0420g	-	YBL	<bmajhd>	-	[Oh.
J06:0420h	-	JJ	EXPERIMENTAL	experimental	.
J06:0420i	-	YBR	<emajhd>	-	.Oh]
J06:0420j	-	YBL	<bminhd>	-	[Oh.
J06:0420k	-	NN2	REAGENTS	reagent	.
J06:0420m	-	YF	+.	-	.
J06:0420n	-	YBR	<eminhd>	-	.Oh]
J06:0420p	-	YD	<mdash>	-	[O.
J06:0430a	-	NP1s	Matheson	Matheson	[S[Ns:S[Ns[Nns.Nns]
J06:0430b	-	JJT	highest	high	[Ns.
J06:0430c	-	NN1u	purity	purity	.Ns]
J06:0430d	-	NN1c	tank	tank	.Ns]
J06:0430e	-	NN1u	chlorine	chlorine	.Ns:S]
J06:0430f	-	VBDZ	was	be	[Vsp.
J06:0430g	-	VVNv	passed	pass	.Vsp]
J06:0430h	-	II	through	through	[P:q.
J06:0430i	-	AT1	a	a	[Ns.
J06:0440a	-	NN1n	tube	tube	.
J06:0440b	-	IO	of	of	[Po.
J06:0440c	-	VVNt	resublimed	resublime	[N[Tn[Vn.Vn]Tn]
J06:0440d	-	FO	<formul>	-	.N]Po]Ns]P:q]
J06:0440e	-	II	into	into	[P:q.
J06:0440f	-	AT1	an	an	[Ns:115.
J06:0440g	-	VVNt	evacuated	evacuate	[Tn[Vn.Vn]Tn]
J06:0440h	-	NP1x	Pyrex	Pyrex	[Nns.Nns]
J06:0440i	-	NN1n	system	system	.
J06:0440j	-	RRQr	where	where	[Fr[Rq:p115.Rq:p115]
J06:0440k	-	PPH1	it	it	[Ni:S.Ni:S]
J06:0440m	-	VBDZ	was	be	[Vsp.
J06:0440n	-	VVNv	condensed	condense	.Vsp]
J06:0450a	-	IW	with	with	[P:h.
J06:0450b	-	NN1n	liquid	liquid	[Ns.
J06:0450c	-	NN1n	air	air	.Ns]P:h]Fr]Ns:115]P:q]S]
J06:0450d	-	YF	+.	-	.
J06:0450e	-	PPH1	It	it	[S[Ni:S.Ni:S]
J06:0450f	-	YG	-	-	[t117.t117]
J06:0450g	-	VBDZ	was	be	[Vsp.
J06:0450h	-	RTn	then	then	[Rsw:G117.Rsw:G117]
J06:0450i	-	VVNv	distilled	distil	.Vsp]
J06:0450j	-	RR21	at	at	[Np:t[RR=.
J06:0450k	-	RR22	least	least	.RR=]
J06:0450m	-	MC	three	three	.
J06:0450n	-	NNT2	times	time	.Np:t]
J06:0460a	-	II	from	from	[P:q.
J06:0460b	-	AT1	a	a	[Ns.
J06:0460c	-	NN1c	trap	trap	.
J06:0460d	-	II	at	at	[P.
J06:0460e	-	MCn	<minus>78	-	[Nu.
J06:0460f	-	NNU	+<deg>	-	.Nu]P]Ns]P:q]
J06:0460g	-	IIt	to	to	[P:q.
J06:0460h	-	AT1	a	a	[Ns.
J06:0460i	-	JJ	liquid	liquid	[Ns.
J06:0460j	-	NN1n	air	air	.Ns]
J06:0460k	-	NN1c	trap	trap	.Ns]P:q]
J06:0460m	-	IW	with	with	[W:b.
J06:0460n	-	RRx	only	only	[Ns:S.
J06:0460p	-	AT1	a	a	.
J06:0460q	-	JJ	small	small	.
J06:0460r	-	NN1c	middle	middle	.
J06:0460s	-	NN1c	fraction	fraction	.Ns:S]
J06:0470a	-	VBG	being	be	[Vgp.
J06:0470b	-	VVNt	retained	retain	.Vgp]
J06:0470c	-	II	in	in	[P:p.
J06:0470d	-	DD1q	each	each	[Ns.
J06:0470e	-	NN1n	distillation	distillation	.Ns]P:p]W:b]S]
J06:0470f	-	YF	+.	-	.
J06:0470g	-	AT	The	the	[S[Ns:S.
J06:0470h	-	VVNt	purified	purify	[Tn[Vn.Vn]Tn]
J06:0470i	-	NN1c	product	product	.Ns:S]
J06:0470j	-	VBDZ	was	be	[Vsp.
J06:0480a	-	VVNt	stored	store	.Vsp]
J06:0480b	-	II	at	at	[P:p.
J06:0480c	-	MCn	<minus>78	-	[Nu.
J06:0480d	-	NNU	+<deg>	-	.Nu]P:p]
J06:0480e	-	II	in	in	[P:p.
J06:0480f	-	AT1	a	a	[Ns:119.
J06:0480g	-	NN1n	tube	tube	.
J06:0480h	-	YG	-	-	[Tn[S119.S119]
J06:0480i	-	VVNt	equipped	equip	[Vn.Vn]
J06:0480j	-	IW	with	with	[P:u.
J06:0480k	-	AT1	a	a	[Ns.
J06:0480m	-	NN1n	break	break	.
J06:0480n	-	NN1c	seal	seal	.Ns]P:u]Tn]Ns:119]P:p]S]
J06:0480p	-	YF	+.	-	.O]
J06:0480q	-	YB	<minbrk>	-	[Oh.Oh]
J06:0480r	-	IO	Of	of	[O[S[Po:G120.
J06:0480s	-	DA2q	several	several	[Np:121.
J06:0490a	-	NN2	methods	method	.
J06:0490b	-	YG	-	-	[Tn[S121.S121]
J06:0490c	-	VVNt	employed	employ	[Vn.Vn]
J06:0490d	-	IF	for	for	[P:c.
J06:0490e	-	VVGv	tagging	tag	[Tg[Vg.Vg]
J06:0490f	-	NN1u	chlorine	chlorine	[Ns:o.Ns:o]
J06:0490g	-	IW	with	with	[P:h.
J06:0490h	-	NN1u	radiochlorine	radiochlorine	.P:h]Tg]P:c]Tn]Np:121]Po:G120]
J06:0490i	-	YC	+,	-	.
J06:0490j	-	AT	the	the	[Ns:S124.
J06:0490k	-	NN1n	exchange	exchange	.
J06:0500a	-	IO	of	of	[Po.
J06:0500b	-	JJ	inactive	inactive	[Ns.
J06:0500c	-	NN1u	chlorine	chlorine	.Ns]Po]
J06:0500d	-	IW	with	with	[P.
J06:0500e	-	VVNv	tagged	tag	[Ns[Tn[Vn.Vn]Tn]
J06:0500f	-	NN1u	aluminum	aluminum	.
J06:0500g	-	NN1u	chloride	chloride	.Ns]P]
J06:0500h	-	II	at	at	[P.
J06:0500i	-	NN1n	room	room	[Ns.
J06:0500j	-	NN1n	temperature	temperature	.Ns]P]Ns:S124]
J06:0510a	-	VBDZ	was	be	[Vsp.
J06:0510b	-	VVNt	found	find	.Vsp]
J06:0510c	-	YG	-	-	[Ti:o[s124.s124]
J06:0510d	-	TO	to	to	[Vib.
J06:0510e	-	VB0	be	be	.Vib]
J06:0510f	-	AT	the	the	[Nj:e.
J06:0510g	-	DAT	most	most	.
J06:0510h	-	JJ	satisfactory	satisfactory	.
J06:0510i	-	YG	-	-	[120.120]Nj:e]Ti:o]S]
J06:0510j	-	YF	+.	-	.
J06:0510k	-	TO	To	to	[S[Ti:c[Vi.
J06:0510m	-	VV0v	prepare	prepare	.Vi]
J06:0510n	-	AT	the	the	[D:o.
J06:0510p	-	DAr	latter	latter	.D:o]Ti:c]
J06:0510q	-	YC	+,	-	.
J06:0520a	-	NN1u	silver	silver	[Ns:S.
J06:0520b	-	NN1u	chloride	chloride	.Ns:S]
J06:0520c	-	VBDZ	was	be	[Vsp.
J06:0520d	-	VVNt	precipitated	precipitate	.Vsp]
J06:0520e	-	II	from	from	[P:q.
J06:0520f	-	AT1	a	a	[Ns:123.
J06:0520g	-	NN1n	solution	solution	.
J06:0520h	-	YG	-	-	[Tg[s123.s123]
J06:0520i	-	VVGt	containing	contain	[Vg.Vg]
J06:0520j	-	FO	<formul>	-	[N:o125.
J06:0520k	-	YG	-	-	[Tn[S125.S125]
J06:0520m	-	VVNv	obtained	obtain	[Vn.Vn]
J06:0530a	-	II	from	from	[P:q.
J06:0530b	-	AT	the	the	[Nns.
J06:0530c	-	NN1n	Oak	oak	[Nns.
J06:0530d	-	NNL1c	Ridge	ridge	.Nns]
J06:0530e	-	JJ	National	national	.
J06:0530f	-	NN1c	Laboratory	laboratory	.Nns]P:q]Tn]N:o125]Tg]Ns:123]P:q]S]
J06:0530g	-	YF	+.	-	.
J06:0530h	-	AT	The	the	[S[Ns:S.
J06:0530i	-	NN1u	silver	silver	.
J06:0530j	-	NN1u	chloride	chloride	.Ns:S]
J06:0530k	-	VBDZ	was	be	[Vsp.
J06:0540a	-	VVNv	fused	fuse	.Vsp]
J06:0540b	-	II	under	under	[P:h.
J06:0540c	-	NN1c	vacuum	vacuum	[Ns.Ns]P:h]
J06:0540d	-	II	in	in	[P:c.
J06:0540e	-	AT	the	the	[Ns.
J06:0540f	-	NN1u	presence	presence	.
J06:0540g	-	IO	of	of	[Po.
J06:0540h	-	NN1u	aluminum	aluminum	[Np.
J06:0540i	-	NN2	chips	chip	.Np]Po]Ns]P:c]
J06:0540j	-	IW	with	with	[P:w.
J06:0540k	-	AT	the	the	[Ns:127.
J06:0540m	-	JJ	resultant	resultant	.
J06:0550a	-	NN1c	product	product	.
J06:0550b	-	IO	of	of	[Po.
J06:0550c	-	FO	<formul>	-	.Po]
J06:0550d	-	DDQr	which	which	[Fr[Dq:S127.Dq:S127]
J06:0550e	-	VBDZ	was	be	[Vsp.
J06:0550f	-	VVNt	sublimed	sublime	.Vsp]
J06:0550g	-	II	into	into	[P:q.
J06:0550h	-	AT1	a	a	[Ns.
J06:0550i	-	NN1c	flask	flask	.
J06:0550j	-	II	on	on	[P.
J06:0550k	-	AT	the	the	[Ns.
J06:0550m	-	NN1c	vacuum	vacuum	.
J06:0550n	-	NN1n	line	line	.Ns]P]Ns]P:q]Fr]Ns:127]P:w]S]
J06:0550p	-	YF	+.	-	.
J06:0560a	-	RR	Previously	previously	[S[Ns:S[Tn[R:t.R:t]
J06:0560b	-	VVNt	purified	purify	[Vn.Vn]Tn]
J06:0560c	-	NN1u	chlorine	chlorine	.Ns:S]
J06:0560d	-	YG	-	-	[t129.t129]
J06:0560e	-	VBDZ	was	be	[Vsp.
J06:0560f	-	RR	subsequently	subsequently	[R:G129.R:G129]
J06:0560g	-	VVNv	admitted	admit	.Vsp]
J06:0560h	-	CC	and	and	[S+.
J06:0560i	-	AT	the	the	[Ns:S131.
J06:0560j	-	NN1n	exchange	exchange	.Ns:S131]
J06:0570a	-	VBDZ	was	be	[Vsp.
J06:0570b	-	VVNv	allowed	allow	.Vsp]
J06:0570c	-	YG	-	-	[Ti:o[s131.s131]
J06:0570d	-	TO	to	to	[Vi.
J06:0570e	-	VV0v	take	take	.Vi]
J06:0570f	-	NNL1c	place	place	[Ns:o.Ns:o]Ti:o]S+]S]
J06:0570g	-	YF	+.	-	.
J06:0570h	-	AT	The	the	[S[Ns:S.
J06:0570i	-	NN1u	radiochlorine	radiochlorine	.Ns:S]
J06:0570j	-	VBDZ	was	be	[Vsp.
J06:0570k	-	VVNt	stored	store	.Vsp]
J06:0570m	-	II	at	at	[P:p.
J06:0570n	-	MCn	<minus>78	-	[Nu.
J06:0570p	-	NNU	+<deg>	-	.Nu]P:p]
J06:0580a	-	II	in	in	[P:p.
J06:0580b	-	AT1	a	a	[Ns:133.
J06:0580c	-	NN1n	tube	tube	.
J06:0580d	-	YG	-	-	[Tn[S133.S133]
J06:0580e	-	VVNt	equipped	equip	[Vn.Vn]
J06:0580f	-	IW	with	with	[P:u.
J06:0580g	-	AT1	a	a	[Ns.
J06:0580h	-	NN1n	break	break	.
J06:0580i	-	NN1c	seal	seal	.Ns]P:u]Tn]Ns:133]P:p]S]
J06:0580j	-	YF	+.	-	.O]
J06:0580k	-	YB	<minbrk>	-	[Oh.Oh]
J06:0580m	-	NNU1c	Liter	litre	[O[S[Np:S.
J06:0580n	-	NN2	quantities	quantity	.
J06:0580p	-	IO	of	of	[Po.
J06:0580q	-	NP1s	Mallinckrodt	Mallinckrodt	[Ns[Nn.
J06:0580r	-	YC	+,	-	.
J06:0590a	-	JJ	low	low	[Ns-.
J06:0590b	-	NN1n	sulfur	sulphur	.Ns-]
J06:0590c	-	YC	+,	-	.
J06:0590d	-	NN1c	reagent	reagent	[Ns-.
J06:0590e	-	NN1c	grade	grade	.Ns-]Nn]
J06:0590f	-	NN1n	carbon	carbon	.
J06:0590g	-	NN1u	tetrachloride	tetrachloride	.Ns]Po]Np:S]
J06:0590h	-	VBDR	were	be	[Vwp.
J06:0590i	-	VVNt	saturated	saturate	.Vwp]
J06:0600a	-	IW	with	with	[P:h.
J06:0600b	-	FO	<formul>	-	[FO&.
J06:0600c	-	CC	and	and	[FO+.
J06:0600d	-	FO	<formul>	-	.FO+]FO&]P:h]
J06:0600e	-	CC	and	and	[S+.
J06:0600f	-	VVNt	illuminated	illuminate	[Vn.Vn]
J06:0600g	-	IF	for	for	[P:t.
J06:0600h	-	RGi	about	about	[Np.
J06:0600i	-	MCn	50	-	.
J06:0600j	-	NNT2	hours	hour	.Np]P:t]
J06:0600k	-	IW	with	with	[P:h.
J06:0600m	-	AT1	a	a	[Ns.
J06:0600n	-	MCn	1000	-	[Nu.
J06:0600p	-	NNU1c	watt	watt	.Nu]
J06:0610a	-	NN1u	tungsten	tungsten	.
J06:0610b	-	NN1c	lamp	lamp	.Ns]P:h]
J06:0610c	-	II	at	at	[P:p.
J06:0610d	-	AT1	a	a	[Ns.
J06:0610e	-	NN1n	distance	distance	.
J06:0610f	-	IO	of	of	[Po.
J06:0610g	-	DD221	a	a	[Nup[DD2=.
J06:0610h	-	DD222	few	few	.DD2=]
J06:0610i	-	NNU2	inches	inch	.Nup]Po]Ns]P:p]S+]S]
J06:0610j	-	YF	+.	-	.
J06:0610k	-	AT	The	the	[S:135[Ns:S.
J06:0610m	-	NN1n	mixture	mixture	.Ns:S]
J06:0610n	-	YG	-	-	[t137.t137]
J06:0610p	-	VBDZ	was	be	[Vsp.
J06:0610q	-	RTn	then	then	[Rsw:G137.Rsw:G137]
J06:0610r	-	VVNt	extracted	extract	.Vsp]
J06:0620a	-	IW	with	with	[P:h.
J06:0620b	-	NN1n	alkali	alkali	.
J06:0620c	-	CC	and	and	[P+.
J06:0620d	-	IW	with	with	.
J06:0620e	-	NNL1n	water	water	.P+]P:h]
J06:0620f	-	II	following	following	[Fr:x[Pq:t.
J06:0620g	-	DDQr	which	which	[Dq:135.Dq:135]Pq:t]
J06:0620h	-	AT	the	the	[Ns:S.
J06:0620i	-	NN1n	carbon	carbon	.
J06:0620j	-	NN1u	tetrachloride	tetrachloride	.Ns:S]
J06:0630a	-	VBDZ	was	be	[Vsp.
J06:0630b	-	VVNv	distilled	distil	.Vsp]
J06:0630c	-	II	on	on	[P:p.
J06:0630d	-	AT1	a	a	[Ns.
J06:0630e	-	NP1s	Vigreux	Vigreux	[Nns.Nns]
J06:0630f	-	NN1c	column	column	.Ns]P:p]
J06:0630g	-	YC	+,	-	.
J06:0630h	-	AT1	a	a	[Tg:b[Ns:S139.
J06:0630i	-	MCn	25	-	[Nu.
J06:0630j	-	NNUp	+%	-	.Nu]
J06:0630k	-	NN1c	center	centre	.
J06:0630m	-	NN1c	cut	cut	.
J06:0630n	-	YG	-	-	[141.141]Ns:S139]
J06:0630p	-	VBG	being	be	[Vgp.
J06:0630q	-	VVNt	retained	retain	.Vgp]
J06:0640a	-	DDQr	which	which	[Fr:G141[Dq:S139.Dq:S139]
J06:0640b	-	YG	-	-	[t143.t143]
J06:0640c	-	VBDZ	was	be	[Vsp.
J06:0640d	-	RTn	then	then	[Rsw:G143.Rsw:G143]
J06:0640e	-	VVNt	degassed	degas	.Vsp]
J06:0640f	-	II	under	under	[P:h.
J06:0640g	-	NN1c	vacuum	vacuum	.P:h]
J06:0640h	-	II	in	in	[P:p.
J06:0640i	-	AT	the	the	[Ns.
J06:0640j	-	NN1u	presence	presence	.
J06:0640k	-	IO	of	of	[Po.
J06:0640m	-	FO	<formul>	-	.Po]Ns]P:p]Fr:G141]Tg:b]Fr:x]S:135]
J06:0640n	-	YF	+.	-	.
J06:0640p	-	VVNt	Purified	purify	[S[Ns:s[Tn[Vn.Vn]Tn]
J06:0650a	-	JJ	inactive	inactive	.
J06:0650b	-	NN1u	chlorine	chlorine	.Ns:s]
J06:0650c	-	YG	-	-	[t145.t145]
J06:0650d	-	VBDZ	was	be	[Vsp.
J06:0650e	-	RTn	then	then	[Rsw:G145.Rsw:G145]
J06:0650f	-	VVNv	added	add	.Vsp]
J06:0650g	-	II	from	from	[P:q.
J06:0650h	-	MC1	one	one	[Ms.
J06:0650i	-	IO	of	of	[Po.
J06:0650j	-	AT	the	the	[Np:147.
J06:0650k	-	NN2	tubes	tube	.
J06:0650m	-	YG	-	-	[Tn[S147.S147]
J06:0650n	-	VVNt	described	describe	[Vn.Vn]
J06:0660a	-	RL	above	above	[R:p.R:p]Tn]Np:147]Po]Ms]P:q]
J06:0660b	-	CC	and	and	[S+.
J06:0660c	-	AT	the	the	[Ns:s.
J06:0660d	-	NN1n	mixture	mixture	.Ns:s]
J06:0660e	-	VVNv	frozen	freeze	[Vn.Vn]
J06:0660f	-	RP	out	out	[R:n.R:n]
J06:0660g	-	CC	and	and	[S+.
J06:0660h	-	VVNv	sealed	seal	[Vn.Vn]
J06:0660i	-	RP	off	off	[R:n.R:n]
J06:0660j	-	II	in	in	[P:p.
J06:0660k	-	AT1	a	a	[Ns:149.
J06:0660m	-	NN1c	flask	flask	.
J06:0660n	-	YG	-	-	[Tn[S149.S149]
J06:0660p	-	VVNt	equipped	equip	[Vn.Vn]
J06:0660q	-	IW	with	with	[P:h.
J06:0670a	-	AT1	a	a	[Ns.
J06:0670b	-	NN1n	break	break	.
J06:0670c	-	NN1c	seal	seal	.Ns]P:h]Tn]Ns:149]P:p]S+]S+]S]
J06:0670d	-	YF	+.	-	.
J06:0670e	-	DD1i	This	this	[S:151[Ns:S.
J06:0670f	-	NN1u	chlorine	chlorine	[N.
J06:0670g	-	YH	+<hyphen>	-	.
J06:0670h	-	NN1n	+carbon	carbon	[Ns.
J06:0670i	-	NN1u	tetrachloride	tetrachloride	.Ns]N]
J06:0670j	-	NN1n	solution	solution	.Ns:S]
J06:0670k	-	VBDZ	was	be	[Vsp.
J06:0670m	-	VVNt	illuminated	illuminate	.Vsp]
J06:0680a	-	IF	for	for	[P:t.
J06:0680b	-	AT1	a	a	[Ns.
J06:0680c	-	NNT1c	day	day	.Ns]P:t]
J06:0680d	-	II	following	following	[Fr:x[Pq:t.
J06:0680e	-	DDQr	which	which	[Dq:151.Dq:151]Pq:t]
J06:0680f	-	AT	the	the	[Ns:S.
J06:0680g	-	NN1c	flask	flask	.Ns:S]
J06:0680h	-	VBDZ	was	be	[Vsp.
J06:0680i	-	VVNt	resealed	reseal	.Vsp]
J06:0680j	-	II	onto	onto	[P:q.
J06:0680k	-	AT1	a	a	[Ns.
J06:0680m	-	NN1c	vacuum	vacuum	.
J06:0690a	-	NN1n	system	system	.Ns]P:q]
J06:0690b	-	CC	and	and	[Fr+.
J06:0690c	-	AT	the	the	[Ns:S.
J06:0690d	-	NN1n	excess	excess	.
J06:0690e	-	NN1u	chlorine	chlorine	.Ns:S]
J06:0690f	-	VVNv	distilled	distil	[Vn.Vn]
J06:0690g	-	RP	off	off	[R:n.R:n]Fr+]Fr:x]S:151]
J06:0690h	-	YF	+.	-	.
J06:0690i	-	AT	The	the	[S[Ns:S.
J06:0690j	-	VVNt	required	require	[Tn[Vn.Vn]Tn]
J06:0690k	-	NN1c	amount	amount	.
J06:0690m	-	IO	of	of	[Po.
J06:0700a	-	NN1n	carbon	carbon	[Ns.
J06:0700b	-	NN1u	tetrachloride	tetrachloride	.Ns]Po]Ns:S]
J06:0700c	-	VBDZ	was	be	[Vsp.
J06:0700d	-	VVNv	distilled	distil	.Vsp]
J06:0700e	-	II	into	into	[P:q.
J06:0700f	-	AT1	a	a	[Ns.
J06:0700g	-	NNc	series	series	.
J06:0700h	-	IO	of	of	[Po.
J06:0700i	-	NN1n	reaction	reaction	[Np.
J06:0700j	-	NN2	cells	cell	.
J06:0700k	-	II	on	on	[P.
J06:0710a	-	AT1	a	a	[Ns.
J06:0710b	-	NN1c	manifold	manifold	.
J06:0710c	-	II	on	on	[P.
J06:0710d	-	AT1	a	a	[Ns.
J06:0710e	-	NN1c	vacuum	vacuum	.
J06:0710f	-	NN1n	line	line	.Ns]P]Ns]P]Np]Po]Ns]P:q]S]
J06:0710g	-	YF	+.	-	.
J06:0710h	-	AT	The	the	[S:153[Np:S.
J06:0710i	-	VVNt	desired	desire	[Tn[Vn.Vn]Tn]
J06:0710j	-	NN2	amounts	amount	.
J06:0710k	-	IO	of	of	[Po.
J06:0710m	-	JJ	inactive	inactive	[N.
J06:0710n	-	NN1u	chlorine	chlorine	.
J06:0720a	-	CC	and	and	[Ns+.
J06:0720b	-	JJ	radioactive	radioactive	.
J06:0720c	-	NN1u	chlorine	chlorine	.Ns+]N]Po]Np:S]
J06:0720d	-	YG	-	-	[h155.h155]
J06:0720e	-	VBDR	were	be	[Vwp.
J06:0720f	-	RR	likewise	likewise	[R:G155.R:G155]
J06:0720g	-	VVNv	condensed	condense	.Vwp]
J06:0720h	-	II	in	in	[P:p.
J06:0720i	-	DD2i	these	these	[Np.
J06:0720j	-	NN2	cells	cell	.
J06:0720k	-	II	on	on	[P.
J06:0730a	-	AT	the	the	[Ns.
J06:0730b	-	NN1c	vacuum	vacuum	.
J06:0730c	-	NN1n	line	line	.Ns]P]Np]P:p]
J06:0730d	-	II	following	following	[Fr:x[Pq:t.
J06:0730e	-	DDQr	which	which	[Dq:153.Dq:153]Pq:t]
J06:0730f	-	PPHS2	they	they	[Nap:S.Nap:S]
J06:0730g	-	VBDR	were	be	[Vwp.
J06:0730h	-	VVNv	frozen	freeze	.Vwp]
J06:0730i	-	RP	down	down	[R:n.R:n]
J06:0730j	-	CC	and	and	[Fr+.
J06:0730k	-	AT	the	the	[Ns:S.
J06:0730m	-	NN1c	manifold	manifold	.
J06:0740a	-	IIa	as	as	[P.
J06:0740b	-	AT1	a	a	[Ns.
J06:0740c	-	NN1c	whole	whole	.Ns]P]Ns:S]
J06:0740d	-	VBDZ	was	be	[Vsp.
J06:0740e	-	VVNv	sealed	seal	.Vsp]
J06:0740f	-	RP	off	off	[R:n.R:n]Fr+]Fr:x]S:153]
J06:0740g	-	YF	+.	-	.
J06:0740h	-	AT	The	the	[S[Np:S.
J06:0740i	-	NN2	contents	content	.
J06:0740j	-	IO	of	of	[Po.
J06:0740k	-	AT	the	the	[Ns.
J06:0740m	-	NN1c	manifold	manifold	.Ns]Po]
J06:0740n	-	IF	for	for	[P.
J06:0740p	-	JJ	liquid	liquid	[Np[Ns.
J06:0740q	-	NN1c	phase	phase	.Ns]
J06:0750a	-	NN2	experiments	experiment	.Np]P]Np:S]
J06:0750b	-	YG	-	-	[t157.t157]
J06:0750c	-	VBDR	were	be	[Vwp.
J06:0750d	-	RTn	then	then	[Rsw:G157.Rsw:G157]
J06:0750e	-	VVNv	mixed	mix	.Vwp]
J06:0750f	-	IIb	by	by	[Pb:h.
J06:0750g	-	VVGv	shaking	shake	[Tg[Vg.Vg]Tg]Pb:h]
J06:0750h	-	YC	+,	-	.
J06:0750i	-	VVNt	redistributed	redistribute	[S-[Vn.Vn]
J06:0750j	-	IIt	to	to	[P:q.
J06:0750k	-	AT	the	the	[Np.
J06:0750m	-	NN1n	reaction	reaction	.
J06:0760a	-	NN2	tubes	tube	.Np]P:q]S-]
J06:0760b	-	YC	+,	-	.
J06:0760c	-	VVNv	frozen	freeze	[S-[Vn.Vn]
J06:0760d	-	RP	down	down	[R:n.R:n]S-]
J06:0760e	-	YC	+,	-	.
J06:0760f	-	CC	and	and	[S+.
J06:0760g	-	DD1q	each	each	[Ns:S.
J06:0760h	-	NN1n	tube	tube	.Ns:S]
J06:0760i	-	YG	-	-	[t159.t159]
J06:0760j	-	VBDZ	was	be	[Vsp.
J06:0760k	-	RTn	then	then	[Rsw:G159.Rsw:G159]
J06:0760m	-	VVNv	sealed	seal	.Vsp]
J06:0760n	-	RP	off	off	[R:n.R:n]S+]S]
J06:0760p	-	YF	+.	-	.
J06:0760q	-	AT	The	the	[S[Np:S161.
J06:0760r	-	NN2	reactants	reactants	.
J06:0770a	-	IF	for	for	[P.
J06:0770b	-	AT	the	the	[Np.
J06:0770c	-	NN1n	gas	gas	[Ns.
J06:0770d	-	NN1c	phase	phase	.Ns]
J06:0770e	-	NN2	experiments	experiment	.Np]P]Np:S161]
J06:0770f	-	YG	-	-	[t163.t163]
J06:0770g	-	VBDR	were	be	[Vwp.
J06:0770h	-	MDo	first	first	[R:G163.R:G163]
J06:0770i	-	VVNv	frozen	freeze	.Vwp]
J06:0770j	-	RP	out	out	[R:n.R:n]
J06:0770k	-	II	in	in	[P:p.
J06:0770m	-	AT1	a	a	[Ns:165.
J06:0770n	-	NN1n	side	side	.
J06:0770p	-	YH	+<hyphen>	-	.
J06:0770q	-	NN1c	+arm	arm	.
J06:0770r	-	YG	-	-	[Tn[S165.S165]
J06:0780a	-	VVNv	attached	attach	[Vn.Vn]
J06:0780b	-	IIt	to	to	[P:q.
J06:0780c	-	AT	the	the	[Ns.
J06:0780d	-	NN1c	manifold	manifold	.Ns]P:q]Tn]Ns:165]P:p]
J06:0780e	-	CC	and	and	[S+.
J06:0780f	-	RTn	then	then	[Rsw:t.Rsw:t]
J06:0780g	-	VVNv	allowed	allow	[Vn.Vn]
J06:0780h	-	YG	-	-	[Ti:o[s161.s161]
J06:0780i	-	TO	to	to	[Vi.
J06:0780j	-	VV0v	distil	distil	.Vi]
J06:0780k	-	RR	slowly	slowly	[R:h.R:h]
J06:0780m	-	II	into	into	[P:q.
J06:0780n	-	AT	the	the	[Ns.
J06:0780p	-	NN1c	manifold	manifold	.
J06:0790a	-	IO	of	of	[Po.
J06:0790b	-	FB	pre	pre<hyphen>	[Np[Tn.
J06:0790c	-	YH	+<hyphen>	-	.
J06:0790d	-	VVNv	+cooled	cool	[Vn.Vn]Tn]
J06:0790e	-	NN1n	reaction	reaction	.
J06:0790f	-	NN2	cells	cell	.Np]Po]Ns]P:q]
J06:0790g	-	ICSt	before	before	[P:t.
J06:0790h	-	VVGv	sealing	seal	[Tg[Vg.Vg]
J06:0790i	-	RP	off	off	[R:n.R:n]Tg]P:t]Ti:o]S+]S]
J06:0790j	-	YF	+.	-	.
J06:0790k	-	DD1i	This	this	[S[Ns:s.
J06:0790m	-	NN1n	method	method	.Ns:s]
J06:0800a	-	RR21	in	in	[R:m[RR=.
J06:0800b	-	RR22	general	general	.RR=]R:m]
J06:0800c	-	VVDt	solved	solve	[Vd.Vd]
J06:0800d	-	AT	the	the	[Ns:o.
J06:0800e	-	NN1c	problem	problem	.
J06:0800f	-	IO	of	of	[Po.
J06:0800g	-	VVGv	obtaining	obtain	[Tg[Vg.Vg]
J06:0800h	-	RR	fairly	fairly	[Np:o[J.
J06:0800i	-	JJ	equal	equal	.J]
J06:0800j	-	NN2	concentrations	concentration	.
J06:0810a	-	IO	of	of	[Po.
J06:0810b	-	NN2	reactants	reactants	.Po]Np:o]
J06:0810c	-	II	in	in	[P:p.
J06:0810d	-	DD1q	each	each	[Ds.
J06:0810e	-	IO	of	of	[Po.
J06:0810f	-	AT	the	the	[Np.
J06:0810g	-	MC	six	six	.
J06:0810h	-	NN2	cells	cell	.
J06:0810i	-	II	from	from	[P.
J06:0810j	-	AT1	a	a	[Ns.
J06:0810k	-	NN1n	set	set	.Ns]P]Np]Po]Ds]P:p]Tg]Po]Ns:o]S]
J06:0810m	-	YF	+.	-	.O]
J06:0810n	-	YBL	<bminhd>	-	[Oh.
J06:0810p	-	NN1n	REACTION	reaction	[N.
J06:0810q	-	NN2	CONDITIONS	condition	.
J06:0820a	-	CC	AND	and	[Ns+.
J06:0820b	-	NN1n	ANALYSIS	analysis	.Ns+]N]
J06:0820c	-	YF	+.	-	.
J06:0820d	-	YBR	<eminhd>	-	.Oh]
J06:0820e	-	YD	<mdash>	-	[O.
J06:0820f	-	AT	The	the	[S[Np:S.
J06:0820g	-	NN2	samples	sample	.
J06:0820h	-	IF	for	for	[P.
J06:0820i	-	JJ	liquid	liquid	[Np[Ns[Ns.
J06:0820j	-	NN1c	phase	phase	.Ns]
J06:0820k	-	JJ	thermal	thermal	.
J06:0820m	-	NN1n	reaction	reaction	.Ns]
J06:0830a	-	NN2	studies	study	.Np]P]Np:S]
J06:0830b	-	VBDR	were	be	[Vwp.
J06:0830c	-	VVNv	prepared	prepare	.Vwp]
J06:0830d	-	II	in	in	[P:p.
J06:0830e	-	NP1x	Pyrex	Pyrex	[Ns[Nns.Nns]
J06:0830f	-	NN1c	capillary	capillary	.
J06:0830g	-	NN1u	tubing	tubing	.
J06:0830h	-	MCd	2.5	-	[N[Nu.
J06:0830i	A	NNU	mm.	-	.Nu]
J06:0830j	A	NN1c	i.d.	-	.
J06:0830k	-	CC	and	and	[Jx+.
J06:0840a	-	RGi	about	about	[Nu.
J06:0840b	-	MCn	15	-	.
J06:0840c	A	NNU	cm.	-	.Nu]
J06:0840d	-	JJ	long	long	.Jx+]N]Ns]P:p]S]
J06:0840e	-	YF	+.	-	.
J06:0840f	-	II	In	in	[S[P:p.
J06:0840g	-	DD221	a	a	[Np[DD2=.
J06:0840h	-	DD222	few	few	.DD2=]
J06:0840i	-	NN2	experiments	experiment	.Np]P:p]
J06:0840j	-	AT	the	the	[Np:S.
J06:0840k	-	NN2	tubes	tube	.Np:S]
J06:0840m	-	VBDR	were	be	[Vwp.
J06:0840n	-	VVNv	made	make	.Vwp]
J06:0840p	-	II	from	from	[P:u.
J06:0850a	-	NN1c	standard	standard	[Ns.
J06:0850b	-	MCn	6	-	[Ns[Nu.
J06:0850c	A	NNU	mm.	-	.Nu]
J06:0850d	A	NN1c	i.d.	-	.Ns]
J06:0850e	-	NP1x	Pyrex	Pyrex	[Nns.Nns]
J06:0850f	-	NN1u	tubing	tubing	.
J06:0850g	-	IO	of	of	[Po.
J06:0850h	-	MC1n	1	-	[Ns[Nu.
J06:0850i	A	NNU	mm.	-	.Nu]
J06:0850j	-	NN1c	wall	wall	.
J06:0850k	-	NN1n	thickness	thickness	.Ns]Po]Ns]P:u]S]
J06:0850m	-	YF	+.	-	.
J06:0850n	-	DB2	Both	both	[S[Np:s.
J06:0860a	-	NN2	types	type	.
J06:0860b	-	IO	of	of	[Po.
J06:0860c	-	NN1n	tube	tube	.Po]Np:s]
J06:0860d	-	VVDt	withstood	withstand	[Vd.Vd]
J06:0860e	-	AT	the	the	[Ns:o167.
J06:0860f	-	NN1n	pressure	pressure	.
J06:0860g	-	IO	of	of	[Po.
J06:0860h	-	RR	approximately	approximately	[Np[M.
J06:0860i	-	MCn	20	-	.M]
J06:0860j	-	NN2	atmospheres	atmosphere	.Np]Po]
J06:0860k	-	YG	-	-	[Tn[S167.S167]
J06:0870a	-	VVNt	exerted	exert	[Vn.Vn]
J06:0870b	-	IIb	by	by	[Pb:a.
J06:0870c	-	AT	the	the	[Ns.
J06:0870d	-	NN1n	carbon	carbon	.
J06:0870e	-	NN1u	tetrachloride	tetrachloride	.Ns]Pb:a]
J06:0870f	-	II	at	at	[P:p.
J06:0870g	-	MCn	220	-	[Nu.
J06:0870h	-	NNU	+<deg>	-	.Nu]P:p]Tn]Ns:o167]S]
J06:0870i	-	YF	+.	-	.
J06:0870j	-	AT	The	the	[S[Np:s.
J06:0870k	-	JJ	photochemical	photochemical	[Ns.
J06:0870m	-	NN1n	reaction	reaction	.Ns]
J06:0880a	-	NN2	cells	cell	.Np:s]
J06:0880b	-	VVDi	consisted	consist	[Vd.Vd]
J06:0880c	-	IO	of	of	[Po:u.
J06:0880d	-	MCn	10	-	[Ns[Ns[Nu.
J06:0880e	A	NNU	mm.	-	.Nu]
J06:0880f	A	NN1c	i.d.	-	.Ns]
J06:0880g	-	NP1x	Pyrex	Pyrex	[Nns.Nns]
J06:0880h	-	NN1u	tubing	tubing	.
J06:0880i	-	YC	+,	-	.
J06:0880j	-	MCd	5.5	-	[Jx[Nu.
J06:0880k	A	NNU	cm.	-	.Nu]
J06:0890a	-	JJ	long	long	.Jx]Ns]Po:u]
J06:0890b	-	YC	+,	-	.
J06:0890c	-	NN1c	diffraction	diffraction	[Tg:b[Np:S.
J06:0890d	-	NN2	effects	effect	.Np:S]
J06:0890e	-	VBG	being	be	[Vgp.
J06:0890f	-	VVNt	minimized	minimize	.Vgp]
J06:0890g	-	IIb	by	by	[Pb:a.
J06:0890h	-	AT	the	the	[Ns.
J06:0890i	-	NN1n	fact	fact	.
J06:0890j	-	CST	that	that	[Fn.
J06:0890k	-	AT	the	the	[Ns:s.
J06:0890m	-	NN1n	light	light	.Ns:s]
J06:0890n	-	VVDv	passed	pass	[Vd.Vd]
J06:0890p	-	YG	-	-	[m168.m168]
J06:0900a	-	II	through	through	[P:q.
J06:0900b	-	RRx	only	only	[R:G168.R:G168]
J06:0900c	-	NN1n	liquid	liquid	[Np[N.
J06:0900d	-	YH	+<hyphen>	-	.
J06:0900e	-	NN1n	+glass	glass	.N]
J06:0900f	-	NN2	interfaces	interface	.
J06:0900g	-	CC	and	and	[Np+.
J06:0900h	-	XX	not	not	.
J06:0900i	-	NN1n	gas	gas	[Ns.
J06:0900j	-	YH	+<hyphen>	-	.
J06:0900k	-	NN1n	+glass	glass	.Ns]
J06:0900m	-	NN2	interfaces	interface	.Np+]Np]P:q]Fn]Ns]Pb:a]Tg:b]S]
J06:0900n	-	YF	+.	-	.
J06:0910a	-	DD2i	These	these	[S[Np:S.
J06:0910b	-	NN2	cells	cell	.Np:S]
J06:0910c	-	VBDR	were	be	[Vwp.
J06:0910d	-	VVNt	used	use	.Vwp]
J06:0910e	-	RRR	rather	rather	[R:m.
J06:0910f	-	CSN	than	than	[P.
J06:0910g	-	JJ	square	square	[Ns.
J06:0910h	-	NP1x	Pyrex	Pyrex	[Nns.Nns]
J06:0910i	-	NN1u	tubing	tubing	.Ns]P]R:m]
J06:0910j	-	II21	because	because	[P:c[II=.
J06:0920a	-	II22	of	of	.II=]
J06:0920b	-	AT	the	the	[Ns.
J06:0920c	-	NN1n	tendency	tendency	.
J06:0920d	-	IO	of	of	[Po.
J06:0920e	-	AT	the	the	[D.
J06:0920f	-	DAr	latter	latter	.D]Po]
J06:0920g	-	TO	to	to	[Ti[Vi.
J06:0920h	-	VV0v	shatter	shatter	.Vi]
J06:0920i	-	CSn	when	when	[Tg:t[Rq:t.Rq:t]
J06:0920j	-	VVGv	thawing	thaw	[Vg.Vg]
J06:0920k	-	VVNv	frozen	freeze	[Ns:o[Tn[Vn.Vn]Tn]
J06:0920m	-	NN1n	carbon	carbon	.
J06:0930a	-	NN1u	tetrachloride	tetrachloride	.Ns:o]Tg:t]Ti]Ns]P:c]S]
J06:0930b	-	YF	+.	-	.
J06:0930c	-	AT	The	the	[S[Np:S.
J06:0930d	-	JJ	round	round	.
J06:0930e	-	NN2	cells	cell	.Np:S]
J06:0930f	-	YG	-	-	[h169.h169]
J06:0930g	-	VBDR	were	be	[Vwp.
J06:0930h	-	RR	reproducibly	reproducibly	[R:G169.R:G169]
J06:0930i	-	VVNt	positioned	position	.Vwp]
J06:0930j	-	II	in	in	[P:p.
J06:0930k	-	AT	the	the	[Ns:171.
J06:0940a	-	NN1n	light	light	.
J06:0940b	-	NN1c	beam	beam	.
J06:0940c	-	DDQr	which	which	[Fr[Dq:s171.Dq:s171]
J06:0940d	-	VVDv	entered	enter	[Vd.Vd]
J06:0940e	-	AT	the	the	[Ns:o.
J06:0940f	-	VVNt	thermostated	thermostat	[Tn[Vn.Vn]Tn]
J06:0940g	-	JJ	mineral	mineral	[Ns.
J06:0940h	-	NN1n	oil	oil	.Ns]
J06:0940i	-	YH	+<hyphen>	-	.
J06:0940j	-	NN1c	+bath	bath	.Ns:o]
J06:0940k	-	II	through	through	[P:q.
J06:0940m	-	AT1	a	a	[Ns.
J06:0940n	-	NN1c	window	window	.Ns]P:q]Fr]Ns:171]P:p]S]
J06:0940p	-	YF	+.	-	.
J06:0950a	-	MC	Two	two	[S[Np:S.
J06:0950b	-	NN2	types	type	.
J06:0950c	-	IO	of	of	[Po.
J06:0950d	-	NN1n	light	light	[Ns.
J06:0950e	-	NN1c	source	source	.
J06:0950f	-	YG	-	-	[172.172]Ns]Po]Np:S]
J06:0950g	-	VBDR	were	be	[Vwp.
J06:0950h	-	VVNt	used	use	.Vwp]
J06:0950i	-	YC	+,	-	.
J06:0950j	-	AT1	a	a	[N@:G172.
J06:0950k	-	NNOc	thousand	thousand	[Nu.
J06:0950m	-	NNU1c	watt	watt	.Nu]
J06:0950n	-	NN1n	projection	projection	.
J06:0960a	-	NN1c	lamp	lamp	.
J06:0960b	-	CC	and	and	[Ns+.
J06:0960c	-	AT1	an	an	.
J06:0960d	S	NP1z	AH5	-	.
J06:0960e	-	JJ	high	high	[Ns.
J06:0960f	-	NN1n	pressure	pressure	.Ns]
J06:0960g	-	NN1u	mercury	mercury	.
J06:0960h	-	NN1c	arc	arc	.Ns+]N@:G172]S]
J06:0960i	-	YF	+.	-	.
J06:0960j	-	AT	The	the	[S[Ns:S.
J06:0960k	-	NN1n	light	light	.Ns:S]
J06:0960m	-	VBDZ	was	be	[Vsp.
J06:0960n	-	VVNv	filtered	filter	.Vsp]
J06:0970a	-	IIb	by	by	[Pb:a.
J06:0970b	-	AT	the	the	[Ns.
J06:0970c	-	JJ	soft	soft	[Ns.
J06:0970d	-	NN1n	glass	glass	.Ns]
J06:0970e	-	NN1c	window	window	.
J06:0970f	-	IO	of	of	[Po.
J06:0970g	-	AT	the	the	[Ns.
J06:0970h	-	NN1c	thermostat	thermostat	.Ns]Po]Ns]Pb:a]
J06:0970i	-	RR	thus	thus	[Tg:c[R:h.R:h]
J06:0970j	-	VVGv	ensuring	ensure	[Vg.Vg]
J06:0970k	-	CST	that	that	[Fn:e.
J06:0980a	-	RRx	only	only	[R:m.R:m]
J06:0980b	-	NN1n	light	light	[Ns:s173.
J06:0980c	-	YG	-	-	[Tn[S173.S173]
J06:0980d	-	VVNt	absorbed	absorb	[Vn.Vn]
J06:0980e	-	IIb	by	by	[Pb:a.
J06:0980f	-	AT	the	the	[Ns.
J06:0980g	-	NN1u	chlorine	chlorine	.Ns]
J06:0980h	-	CC	and	and	[Pb+.
J06:0980i	-	XX	not	not	.
J06:0980j	-	IIb	by	by	.
J06:0980k	-	AT	the	the	[Ns.
J06:0980m	-	NN1n	carbon	carbon	.
J06:0980n	-	NN1u	tetrachloride	tetrachloride	.Ns]Pb+]Pb:a]Tn]Ns:s173]
J06:0990a	-	VMd	could	can	[Vdc.
J06:0990b	-	VV0v	enter	enter	.Vdc]
J06:0990c	-	AT	the	the	[Ns:o.
J06:0990d	-	NN1n	reaction	reaction	.
J06:0990e	-	NN1c	cell	cell	.Ns:o]Fn:e]Tg:c]S]
J06:0990f	-	YF	+.	-	.
J06:0990g	-	JJ	Relative	relative	[S[Np:S.
J06:0990h	-	NN1c	incident	incident	[Ns.
J06:0990i	-	NN1n	light	light	.Ns]
J06:0990j	-	NN2	intensities	intensity	.Np:S]
J06:1000a	-	VBDR	were	be	[Vwp.
J06:1000b	-	VVNv	measured	measure	.Vwp]
J06:1000c	-	IW	with	with	[P:h.
J06:1000d	-	AT1	a	a	[Ns.
J06:1000e	-	NN1c	thermopile	thermopile	[Ns.
J06:1000f	-	NN1c	potentiometer	potentiometer	.Ns]
J06:1000g	-	NN1n	system	system	.Ns]P:h]S]
J06:1000h	-	YF	+.	-	.
J06:1000i	-	NN2	Changes	change	[S[Np:S.
J06:1000j	-	IO	of	of	[Po.
J06:1000k	-	NN1n	intensity	intensity	.Po]
J06:1010a	-	II	on	on	[P.
J06:1010b	-	AT	the	the	[Ns.
J06:1010c	-	NN1c	cell	cell	.Ns]P]Np:S]
J06:1010d	-	VBDR	were	be	[Vwp.
J06:1010e	-	VVNt	achieved	achieve	.Vwp]
J06:1010f	-	IIb	by	by	[Pb:a.
J06:1010g	-	NN1n	use	use	[N.
J06:1010h	-	IO	of	of	[Po.
J06:1010i	-	AT1	a	a	[Ns.
J06:1010j	-	NN1n	wire	wire	.
J06:1010k	-	NN1c	screen	screen	.Ns]Po]
J06:1010m	-	CC	and	and	[Pb+.
J06:1010n	-	IIb	by	by	.
J06:1010p	-	VVGv	varying	vary	[Tg[Vg.Vg]
J06:1020a	-	AT	the	the	[Ns:o.
J06:1020b	-	NN1n	distance	distance	.
J06:1020c	-	IO	of	of	[Po.
J06:1020d	-	AT	the	the	[Ns.
J06:1020e	-	NN1n	light	light	.
J06:1020f	-	NN1c	source	source	.Ns]Po]
J06:1020g	-	II	from	from	[P.
J06:1020h	-	AT	the	the	[Ns.
J06:1020i	-	NN1c	cell	cell	.Ns]P]Ns:o]Tg]Pb+]N]Pb:a]S]
J06:1020j	-	YF	+.	-	.O]
J06:1020k	-	YB	<minbrk>	-	[Oh.Oh]
J06:1020m	-	II	Following	following	[O[S[P:t.
J06:1020n	-	NN1n	reaction	reaction	.P:t]
J06:1030a	-	AT	the	the	[Np:S.
J06:1030b	-	NN2	cells	cell	.Np:S]
J06:1030c	-	VBDR	were	be	[Vwp.
J06:1030d	-	VVNv	scratched	scratch	.Vwp]
J06:1030e	-	IW	with	with	[P:h.
J06:1030f	-	AT1	a	a	[Ns.
J06:1030g	-	NN1c	file	file	.Ns]P:h]
J06:1030h	-	CC	and	and	[S+.
J06:1030i	-	VVDv	opened	open	[Vd.Vd]
J06:1030j	-	II	under	under	[P:p.
J06:1030k	-	AT1	a	a	[Ns.
J06:1030m	-	MCn	20	-	[Nu.
J06:1030n	-	NNUp	+%	-	.Nu]
J06:1030p	-	JJ	aqueous	aqueous	.
J06:1040a	-	NN1u	sodium	sodium	[Ns.
J06:1040b	-	NN1u	iodide	iodide	.Ns]
J06:1040c	-	NN1n	solution	solution	.Ns]P:p]S+]S]
J06:1040d	-	YF	+.	-	.
J06:1040e	-	NN1c	Carrier	carrier	[S[Ns:S.
J06:1040f	-	FO	<formul>	-	.Ns:S]
J06:1040g	-	VBDZ	was	be	[Vsp.
J06:1040h	-	VVNv	added	add	.Vsp]
J06:1040i	-	CC	and	and	[S+.
J06:1040j	-	AT	the	the	[Np:S.
J06:1040k	-	JJ	aqueous	aqueous	[JJ&.
J06:1040m	-	CC	and	and	[JJ+.
J06:1050a	-	JJ	organic	organic	.JJ+]JJ&]
J06:1050b	-	NN2	phases	phase	.Np:S]
J06:1050c	-	VBDR	were	be	[Vwp.
J06:1050d	-	VVNv	separated	separate	.Vwp]
J06:1050e	-	YPL	(	-	.
J06:1050f	-	NN2	+cells	cell	[I[S[Np:S175.
J06:1050g	-	YG	-	-	[Tg[s175.s175]
J06:1050h	-	VVGt	containing	contain	[Vg.Vg]
J06:1050i	-	JJ	gaseous	gaseous	[Np:o.
J06:1050j	-	NN2	reactants	reactants	.Np:o]Tg]Np:S175]
J06:1050k	-	VBDR	were	be	[Vwp.
J06:1060a	-	VVNt	immersed	immerse	.Vwp]
J06:1060b	-	II	in	in	[P:q.
J06:1060c	-	JJ	liquid	liquid	[Ns.
J06:1060d	-	NN1n	air	air	.Ns]P:q]
J06:1060e	-	ICSt	before	before	[Fa:t.
J06:1060f	-	VVGv	opening	open	[Vg.Vg]
J06:1060g	-	II	under	under	[P:p.
J06:1060h	-	NN1u	sodium	sodium	[Ns.
J06:1060i	-	NN1u	iodide	iodide	.Ns]P:p]Fa:t]S]I]
J06:1060j	-	YPR	+)	-	.S+]S]
J06:1060k	-	YF	+.	-	.
J06:1060m	-	ICSt	After	after	[S[P:t.
J06:1070a	-	NN1n	titration	titration	[Ns.
J06:1070b	-	IO	of	of	[Po.
J06:1070c	-	AT	the	the	[N.
J06:1070d	-	VVNt	liberated	liberate	[Tn[Vn.Vn]Tn]
J06:1070e	-	FO	<formul>	-	.N]Po]
J06:1070f	-	IW	with	with	[P.
J06:1070g	-	FO	<formul>	-	.P]Ns]P:t]
J06:1070h	-	YC	+,	-	.
J06:1070i	-	NN2	aliquots	aliquots	[Np:S.
J06:1070j	-	IO	of	of	[Po.
J06:1070k	-	AT	the	the	[N.
J06:1070m	-	JJ	aqueous	aqueous	.
J06:1070n	-	CC	and	and	[Po+.
J06:1071a	-	IO	of	of	.
J06:1071b	-	AT	the	the	[N.
J06:1071c	-	JJ	organic	organic	.N]Po+]
J06:1080a	-	NN1c	phase	phase	.N]Po]Np:S]
J06:1080b	-	VBDR	were	be	[Vwp.
J06:1080c	-	VVNv	counted	count	.Vwp]
J06:1080d	-	II	in	in	[P:p.
J06:1080e	-	AT1	a	a	[Ns.
J06:1080f	-	NN1n	solution	solution	[J.
J06:1080g	-	YH	+<hyphen>	-	.
J06:1080h	-	FA	+type	type	.J]
J06:1080i	-	NP1s	Geiger	Geiger	[Nns.Nns]
J06:1080j	-	NN1n	tube	tube	.Ns]P:p]S]
J06:1080k	-	YF	+.	-	.
J06:1080m	-	II	In	in	[S[P:p.
J06:1080n	-	AT	the	the	[Np.
J06:1080p	-	JJ	liquid	liquid	[Ns.
J06:1090a	-	NN1c	phase	phase	.Ns]
J06:1090b	-	NN2	runs	run	.Np]P:p]
J06:1090c	-	AT	the	the	[Ns:S.
J06:1090d	-	NN1c	amount	amount	.
J06:1090e	-	IO	of	of	[Po.
J06:1090f	-	NN1n	carbon	carbon	[Ns.
J06:1090g	-	NN1u	tetrachloride	tetrachloride	.Ns]Po]
J06:1090h	-	II	in	in	[P.
J06:1090i	-	DD1q	each	each	[Ns.
J06:1090j	-	NN1n	reaction	reaction	.
J06:1090k	-	NN1n	tube	tube	.Ns]P]Ns:S]
J06:1090m	-	VBDZ	was	be	[Vsp.
J06:1100a	-	VVNv	determined	determine	.Vsp]
J06:1100b	-	IIb	by	by	[Pb:a.
J06:1100c	-	VVGv	weighing	weigh	[Tg[Vg.Vg]
J06:1100d	-	AT	the	the	[Ns:o.
J06:1100e	-	NN1n	tube	tube	.Ns:o]
J06:1100f	-	ICSt	before	before	[Fa:t.
J06:1100g	-	VVGv	opening	open	[Vg.Vg]
J06:1100h	-	CC	and	and	[Fa+.
J06:1100i	-	VVGv	weighing	weigh	[Vg.Vg]
J06:1100j	-	AT	the	the	[Np:o.
J06:1100k	-	NN2	fragments	fragment	.Np:o]
J06:1110a	-	ICSt	after	after	[Fa:t.
J06:1110b	-	VVGv	emptying	empty	[Vg.Vg]Fa:t]Fa+]Fa:t]Tg]Pb:a]S]
J06:1110c	-	YF	+.	-	.
J06:1110d	-	AT	The	the	[S[Ns:S.
J06:1110e	-	NN1c	fraction	fraction	.
J06:1110f	-	IO	of	of	[Po.
J06:1110g	-	NN1n	exchange	exchange	.Po]Ns:S]
J06:1110h	-	VBDZ	was	be	[Vsp.
J06:1110i	-	VVNv	determined	determine	.Vsp]
J06:1110j	-	IIa	as	as	[P:e.
J06:1110k	-	AT	the	the	[Ns.
J06:1120a	-	NN1c	ratio	ratio	.
J06:1120b	-	IO	of	of	[Po.
J06:1120c	-	AT	the	the	[Np:177.
J06:1120d	-	NNS2	counts	count	.
J06:1120e	-	IIp	+<sol>	-	[P.
J06:1120f	-	NNT1c	+minute	minute	.P]
J06:1120g	-	YG	-	-	[Tn[S177.S177]
J06:1120h	-	VVNv	observed	observe	[Vn.Vn]
J06:1120i	-	II	in	in	[P:p.
J06:1120j	-	AT	the	the	[Ns.
J06:1120k	-	NN1n	carbon	carbon	.
J06:1120m	-	NN1u	tetrachloride	tetrachloride	.Ns]P:p]Tn]Np:177]Po]
J06:1120n	-	IIt	to	to	[P.
J06:1120p	-	AT	the	the	[Np:179.
J06:1130a	-	NNS2	counts	count	.
J06:1130b	-	IIp	+<sol>	-	[P.
J06:1130c	-	NNT1c	+minute	minute	.P]
J06:1130d	-	YG	-	-	[Tn[S179.S179]
J06:1130e	-	VVNv	calculated	calculate	[Vn.Vn]
J06:1130f	-	IF	for	for	[P:r.
J06:1130g	-	AT	the	the	[Np.
J06:1130h	-	NN1n	carbon	carbon	[Ns.
J06:1130i	-	NN1u	tetrachloride	tetrachloride	.Ns]
J06:1130j	-	NN2	fractions	fraction	.Np]P:r]
J06:1130k	-	IF	for	for	[P:r.
J06:1140a	-	NN1u	equilibrium	equilibrium	[Ns.
J06:1140b	-	NN1n	distribution	distribution	.
J06:1140c	-	IO	of	of	[Po.
J06:1140d	-	AT	the	the	[Ns.
J06:1140e	-	NN1n	activity	activity	.Ns]Po]
J06:1140f	-	II	between	between	[P.
J06:1140g	-	AT	the	the	[N.
J06:1140h	-	NN1u	chlorine	chlorine	.
J06:1140i	-	CC	and	and	[Ns+.
J06:1140j	-	NN1n	carbon	carbon	.
J06:1150a	-	NN1u	tetrachloride	tetrachloride	.Ns+]N]P]Ns]P:r]Tn]Np:179]P]Ns]P:e]
J06:1150b	-	YC	+,	-	.
J06:1150c	-	RR	empirically	empirically	[Tg:b[Ns:S[Tn[R:h.R:h]
J06:1150d	-	VVNv	determined	determine	[Vn.Vn]Tn]
J06:1150e	-	NN1n	correction	correction	.Ns:S]
J06:1150f	-	VBG	being	be	[Vgp.
J06:1150g	-	VVNv	made	make	.Vgp]
J06:1150h	-	IF	for	for	[P:c.
J06:1150i	-	AT	the	the	[Ns.
J06:1160a	-	NN1n	difference	difference	.
J06:1160b	-	II	in	in	[P.
J06:1160c	-	VVGv	counting	count	[Ns[Tg[Vg.Vg]Tg]
J06:1160d	-	NN1u	efficiency	efficiency	.
J06:1160e	-	IO	of	of	[Po.
J06:1160f	-	FO	<formul>	-	.Po]Ns]P]
J06:1160g	-	II	in	in	[P.
J06:1160h	-	FO	<formul>	-	[FO&.
J06:1160i	-	CC	and	and	[FO+.
J06:1160j	-	FO	<formul>	-	.FO+]FO&]P]Ns]P:c]Tg:b]S]
J06:1160k	-	YF	+.	-	.O]
J06:1160m	-	YBL	<bmajhd>	-	[Oh.
J06:1160n	-	NN2	RESULTS	result	.
J06:1160p	-	YBR	<emajhd>	-	.Oh]
J06:1170a	-	YBL	<bminhd>	-	[Oh.
J06:1170b	-	AT	THE	the	[Ns.
J06:1170c	-	JJ	THERMAL	thermal	.
J06:1170d	-	NN1n	REACTION	reaction	.Ns]
J06:1170e	-	YF	+.	-	.
J06:1170f	-	YBR	<eminhd>	-	.Oh]
J06:1170g	-	YD	<mdash>	-	[O.
J06:1170h	-	II	In	in	[S[P:p.
J06:1170i	-	VVGv	studying	study	[Tg[Vg.Vg]
J06:1170j	-	AT	the	the	[Ns:o.
J06:1170k	-	JJ	liquid	liquid	[Ns.
J06:1170m	-	NN1c	phase	phase	.Ns]
J06:1170n	-	JJ	thermal	thermal	.
J06:1180a	-	NN1n	reaction	reaction	.Ns:o]Tg]P:p]
J06:1180b	-	YC	+,	-	.
J06:1180c	-	DDi	some	some	[Np:S[M.
J06:1180d	-	MCn	70	-	.M]
J06:1180e	-	NN2	tubes	tube	.
J06:1180f	-	II	from	from	[P.
J06:1180g	-	MCn	12	-	[Np.
J06:1180h	-	JJ	different	different	.
J06:1180i	-	NN1c	manifold	manifold	.
J06:1180j	-	NN2	fillings	filling	.Np]P]Np:S]
J06:1180k	-	VBDR	were	be	[Vwp.
J06:1180m	-	VVNv	prepared	prepare	.Vwp]
J06:1190a	-	CC	and	and	[S+.
J06:1190b	-	VVNt	analyzed	analyze	[Vn.Vn]S+]S]
J06:1190c	-	YF	+.	-	.
J06:1190d	-	NN2	Experiments	experiment	[S[Np:s.Np:s]
J06:1190e	-	VBDR	were	be	[Vwp.
J06:1190f	-	VDN	done	do	.Vwp]
J06:1190g	-	II	at	at	[P:p.
J06:1190h	-	MCn	180	-	[Nu[MCn&.
J06:1190i	-	YC	+,	-	.
J06:1190j	-	MCn	200	-	[MCn-.MCn-]
J06:1190k	-	YC	+,	-	.
J06:1190m	-	MCn	210	-	[MCn-.MCn-]
J06:1190n	-	YC	+,	-	.
J06:1190p	-	MCn	220	-	[MCn-.MCn-]MCn&]
J06:1190q	-	NNU	+<deg>	-	.Nu]P:p]S]
J06:1190r	-	YF	+.	-	.
J06:1190s	-	II	Following	following	[S[P:t.
J06:1200a	-	NN1n	observation	observation	[Ns.
J06:1200b	-	IO	of	of	[Po.
J06:1200c	-	AT	the	the	[Ns.
J06:1200d	-	NN1n	fact	fact	.
J06:1200e	-	CST	that	that	[Fn.
J06:1200f	-	AT	the	the	[Np:s.
J06:1200g	-	NN1n	reaction	reaction	.
J06:1200h	-	NN2	rates	rate	.
J06:1200i	-	IO	of	of	[Po.
J06:1200j	-	RR	supposedly	supposedly	[Np:181[J.
J06:1210a	-	JJ	identical	identical	.J]
J06:1210b	-	NN1n	reaction	reaction	.
J06:1210c	-	NN2	mixtures	mixture	.
J06:1210d	-	YG	-	-	[Tn[S181.S181]
J06:1210e	-	VVNv	prepared	prepare	[Vn.Vn]
J06:1210f	-	II	on	on	[P:p.
J06:1210g	-	AT	the	the	[Ns.
J06:1210h	-	DAy	same	same	.
J06:1210i	-	NN1n	filling	filling	.
J06:1210j	-	NN1c	manifold	manifold	.Ns]P:p]
J06:1210k	-	CC	and	and	[Tn+.
J06:1220a	-	VVNt	exposed	expose	[Vn.Vn]
J06:1220b	-	II	under	under	[P:h.
J06:1220c	-	JJ	identical	identical	[Np.
J06:1220d	-	NN2	conditions	condition	.Np]P:h]Tn+]Tn]Np:181]Po]Np:s]
J06:1220e	-	RR	often	often	[R:t.R:t]
J06:1220f	-	VVDi	differed	differ	[Vd.Vd]
J06:1220g	-	IIb	by	by	[Pb:h.
J06:1220h	-	DA2q	several	several	[Nu[M.
J06:1220i	-	NNOc	hundred	hundred	.M]
J06:1220j	-	NNUp21	per	per	[NNUp=.
J06:1230a	A	NNUp22	cent.	-	.NNUp=]Nu]Pb:h]Fn]Ns]Po]Ns]P:t]
J06:1230b	-	YC	+,	-	.
J06:1230c	-	AT1	a	a	[Ns:S.
J06:1230d	-	JJ	systematic	systematic	.
J06:1230e	-	NNc	series	series	.
J06:1230f	-	IO	of	of	[Po.
J06:1230g	-	NN2	experiments	experiment	.Po]Ns:S]
J06:1230h	-	VBDZ	was	be	[Vsp.
J06:1230i	-	VVNt	undertaken	undertake	.Vsp]
J06:1230j	-	TO	to	to	[Ti:c[Vi.
J06:1230k	-	VV0v	see	see	.Vi]
J06:1230m	-	CSW	whether	whether	[Fn?:o.
J06:1240a	-	AT	the	the	[Ns:S.
J06:1240b	-	NN1n	difficulty	difficulty	.Ns:S]
J06:1240c	-	VMd	could	can	[Vdcp.
J06:1240d	-	VB0	be	be	.
J06:1240e	-	VVNt	ascribed	ascribe	.Vdcp]
J06:1240f	-	IIt	to	to	[P:u.
J06:1240g	-	AT	the	the	[Ns.
J06:1240h	-	NN1n	method	method	.
J06:1240i	-	IO	of	of	[Po.
J06:1240j	-	VVGv	preparing	prepare	[Tg[Vg.Vg]
J06:1240k	-	AT	the	the	[Ns:o.
J06:1240m	-	NN1u	chlorine	chlorine	.Ns:o]Tg]Po]Ns]
J06:1240n	-	YC	+,	-	.
J06:1250a	-	IIt	to	to	[P-.
J06:1250b	-	AT	the	the	[Np.
J06:1250c	-	NN2	effects	effect	.
J06:1250d	-	IO	of	of	[Po.
J06:1250e	-	NN1u	oxygen	oxygen	[NN1u&.
J06:1250f	-	CCr	or	or	[NN1u+.
J06:1250g	-	NN1u	moisture	moisture	.NN1u+]NN1u&]Po]Np]P-]
J06:1250h	-	CCr	or	or	[P+.
J06:1250i	-	IIt	to	to	.
J06:1250j	-	AT	the	the	[Ns.
J06:1250k	-	NN1n	effect	effect	.
J06:1250m	-	IO	of	of	[Po.
J06:1250n	-	NN1c	surface	surface	[Ns[Ns.
J06:1260a	-	IIt	to	to	[P.
J06:1260b	-	NN1n	volume	volume	.P]Ns]
J06:1260c	-	NN1c	ratio	ratio	.
J06:1260d	-	II	in	in	[P.
J06:1260e	-	AT	the	the	[Np.
J06:1260f	-	NN1n	reaction	reaction	.
J06:1260g	-	NN2	tubes	tube	.Np]P]Ns]Po]Ns]P+]P:u]Fn?:o]Ti:c]S]
J06:1260h	-	YF	+.	-	.
J06:1260i	-	II	In	in	[S[P:m.
J06:1260j	-	NN1n	addition	addition	[Ns.
J06:1260k	-	IIt	to	to	[P.
J06:1260m	-	AT	the	the	[Ns:183.
J06:1260n	-	NN1n	method	method	.
J06:1260p	-	YG	-	-	[Tn[S183.S183]
J06:1270a	-	VVNt	described	describe	[Vn.Vn]
J06:1270b	-	II	in	in	[P:p.
J06:1270c	-	AT	the	the	[Ns.
J06:1270d	-	NN1c	section	section	.
J06:1270e	-	RL	above	above	.Ns]P:p]Tn]Ns:183]P]Ns]P:m]
J06:1270f	-	YC	+,	-	.
J06:1270g	-	NN1u	chlorine	chlorine	[N:S[NN1u&.
J06:1270h	-	CC	and	and	[NN1u+.
J06:1270i	-	NN1u	radiochlorine	radiochlorine	.NN1u+]NN1u&]N:S]
J06:1270j	-	VBDR	were	be	[Vwp.
J06:1270k	-	VVNv	prepared	prepare	.Vwp]
J06:1280a	-	IIb	by	by	[Pb:h.
J06:1280b	-	AT	the	the	[Ns.
J06:1280c	-	NN1u	electrolysis	electrolysis	.
J06:1280d	-	IO	of	of	[Po.
J06:1280e	-	AT1	a	a	[Ns.
J06:1280f	-	FO	<formul>	-	.
J06:1280g	-	NN1n	eutectic	eutectic	.Ns]Po]
J06:1280h	-	II	on	on	[P.
J06:1280i	-	AT	the	the	[Ns.
J06:1280j	-	NN1c	vacuum	vacuum	.
J06:1280k	-	NN1n	line	line	.Ns]P]Ns]
J06:1280m	-	YC	+,	-	.
J06:1280n	-	CC	and	and	[Pb+.
J06:1280p	-	IIb	by	by	.
J06:1280q	-	NN1n	exchange	exchange	[Ns.
J06:1290a	-	IO	of	of	[Po.
J06:1290b	-	FO	<formul>	-	.Po]
J06:1290c	-	IW	with	with	[P.
J06:1290d	-	VVNv	molten	melt	[N[Tn[Vn.Vn]Tn]
J06:1290e	-	FO	<formul>	-	.N]P]Ns]Pb+]Pb:h]S]
J06:1290f	-	YF	+.	-	.
J06:1290g	-	NN1u	Calcium	calcium	[S[Ns:S.
J06:1290h	-	NN1u	hydride	hydride	.Ns:S]
J06:1290i	-	VBDZ	was	be	[Vsp.
J06:1290j	-	VVNv	substituted	substitute	.Vsp]
J06:1290k	-	IF	for	for	[P:u.
J06:1290m	-	FO	<formul>	-	.P:u]
J06:1300a	-	IIa	as	as	[P:e.
J06:1300b	-	AT1	a	a	[Ns.
J06:1300c	-	VVGv	drying	dry	[Tg[Vg.Vg]Tg]
J06:1300d	-	NN1c	agent	agent	.
J06:1300e	-	IF	for	for	[P.
J06:1300f	-	NN1n	carbon	carbon	[Ns.
J06:1300g	-	NN1u	tetrachloride	tetrachloride	.Ns]P]Ns]P:e]S]
J06:1300h	-	YF	+.	-	.
J06:1300i	-	ATn	No	no	[S[Ns:S.
J06:1300j	-	NN1c	correlation	correlation	.
J06:1300k	-	II	between	between	[P.
J06:1310a	-	DD2i	these	these	[N.
J06:1310b	-	NN2	variables	variable	.
J06:1310c	-	CC	and	and	[Ns+.
J06:1310d	-	AT	the	the	.
J06:1310e	-	NN1u	irreproducibility	irreproducibility	.
J06:1310f	-	IO	of	of	[Po.
J06:1310g	-	AT	the	the	[Np.
J06:1310h	-	NN2	results	result	.Np]Po]Ns+]N]P]Ns:S]
J06:1310i	-	VBDZ	was	be	[Vsp.
J06:1310j	-	VVNt	found	find	.Vsp]S]
J06:1310k	-	YF	+.	-	.O]
J06:1320a	-	YB	<minbrk>	-	[Oh.Oh]
J06:1320b	-	AT	The	the	[O[S[Np:s185.
J06:1320c	-	NN1n	reaction	reaction	.
J06:1320d	-	NN2	rates	rate	.
J06:1320e	-	YG	-	-	[Tn[S185.S185]
J06:1320f	-	VVNv	observed	observe	[Vn.Vn]
J06:1320g	-	II	at	at	[P:p.
J06:1320h	-	MCn	200	-	[Nu.
J06:1320i	-	NNU	+<deg>	-	.Nu]P:p]Tn]Np:s185]
J06:1320j	-	VVDv	ranged	range	[Vd.Vd]
J06:1320k	-	II	from	from	[P:q.
J06:1320m	-	FO	<formul>	-	[Tn[N:S.
J06:1320n	-	IO	of	of	[Po.
J06:1320p	-	AT	the	the	[Ns.
J06:1320q	-	NN1u	chlorine	chlorine	.Ns]Po]N:S]
J06:1330a	-	VVNt	exchanged	exchange	[Vn.Vn]
J06:1330b	-	IIp	per	per	[P:t.
J06:1330c	-	NNT1c	hour	hour	.P:t]Tn]P:q]
J06:1330d	-	IIt	to	to	[P:q.
J06:1330e	-	MCd	0.7	-	[Tn[M:S.M:S]
J06:1330f	-	VVNt	exchanged	exchange	[Vn.Vn]
J06:1330g	-	IIp	per	per	[P:t.
J06:1330h	-	NNT1c	hour	hour	.P:t]Tn]P:q]S]
J06:1330i	-	YF	+.	-	.
J06:1330j	-	II	In	in	[S[P:m.
J06:1330k	-	DAT	most	most	[Np.
J06:1330m	-	NN2	cases	case	.Np]P:m]
J06:1330n	-	AT	the	the	[Ns:s.
J06:1331a	-	NN1u	chlorine	chlorine	.
J06:1340a	-	NN1n	concentration	concentration	.Ns:s]
J06:1340b	-	VBDZ	was	be	[Vsb.Vsb]
J06:1340c	-	RGi	about	about	[N:e.
J06:1340d	-	FO	<formul>	-	.N:e]S]
J06:1340e	-	YF	+.	-	.
J06:1340f	-	NN2	Sets	set	[S[Np:s191.
J06:1340g	-	IO	of	of	[Po.
J06:1340h	-	NN1n	reaction	reaction	[Np.
J06:1340i	-	NN2	tubes	tube	.Np]Po]
J06:1340j	-	YG	-	-	[Tg[s191.s191]
J06:1340k	-	VVGt	containing	contain	[Vg.Vg]
J06:1340m	-	MCd	0.2	-	[M:o.
J06:1340n	-	IO	of	of	[Po.
J06:1350a	-	AT1	an	an	[Ns.
J06:1350b	-	NN1n	atmosphere	atmosphere	.Ns]Po]
J06:1350c	-	IO	of	of	[Po.
J06:1350d	-	VVNv	added	add	[Ns[Tn[Vn.Vn]Tn]
J06:1350e	-	NN1u	oxygen	oxygen	.Ns]Po]M:o]
J06:1350f	-	II	in	in	[P:r.
J06:1350g	-	MC1	one	one	[Ns.
J06:1350h	-	NN1c	case	case	.Ns]P:r]
J06:1350i	-	CC	and	and	[Tg+.
J06:1350j	-	VVNv	added	add	[Ns:o[Tn[Vn.Vn]Tn]
J06:1350k	-	NN1u	moisture	moisture	.Ns:o]
J06:1350m	-	II	in	in	[P:r.
J06:1350n	-	DD1q	another	another	.P:r]Tg+]Tg]Np:s191]
J06:1350p	-	YC	+,	-	.
J06:1360a	-	RR	both	both	[R:h.R:h]
J06:1360b	-	VVDv	gave	give	[Vd.Vd]
J06:1360c	-	NN1n	reaction	reaction	[Np:o.
J06:1360d	-	NN2	rates	rate	.
J06:1360e	-	II	in	in	[P.
J06:1360f	-	AT	the	the	[Ns.
J06:1360g	-	NN1c	range	range	.
J06:1360h	-	IO	of	of	[Po.
J06:1360i	-	MCd	0.1	-	[Tn[M:S.
J06:1360j	-	IIt	to	to	[P.
J06:1360k	-	MCd	0.4	-	.P]
J06:1360m	-	IO	of	of	[Po.
J06:1360n	-	AT	the	the	[Ns.
J06:1360p	-	NN1u	chlorine	chlorine	.Ns]Po]M:S]
J06:1370a	-	VVNt	exchanged	exchange	[Vn.Vn]
J06:1370b	-	IIp	per	per	[P:t.
J06:1370c	-	NNT1c	hour	hour	.P:t]Tn]Po]Ns]P]Np:o]S]
J06:1370d	-	YF	+.	-	.
J06:1370e	-	ATn	No	no	[S[Ns:S.
J06:1370f	-	JJ	detectable	detectable	.
J06:1370g	-	NN1n	reaction	reaction	.Ns:S]
J06:1370h	-	VBDZ	was	be	[Vsp.
J06:1370i	-	VVNt	found	find	.Vsp]
J06:1370j	-	II	at	at	[P:p.
J06:1370k	-	NN1n	room	room	[Ns.
J06:1370m	-	NN1n	temperature	temperature	.Ns]P:p]
J06:1380a	-	IF	for	for	[P:r.
J06:1380b	-	NN1n	reaction	reaction	[Np:195.
J06:1380c	-	NN2	mixtures	mixture	.
J06:1380d	-	YG	-	-	[Tn[S195.S195]
J06:1380e	-	VVNv	allowed	allow	[Vn.Vn]
J06:1380f	-	YG	-	-	[Ti:o[s195.s195]
J06:1380g	-	TO	to	to	[Vi.
J06:1380h	-	VV0v	stand	stand	.Vi]
J06:1380i	-	RGi21	up	up	[Np:t[RGi=.
J06:1380j	-	RGi22	to	to	.RGi=]
J06:1380k	-	MCn	5	-	.
J06:1380m	-	NNT2	hours	hour	.Np:t]Ti:o]Tn]Np:195]P:r]S]
J06:1380n	-	YF	+.	-	.O]
J06:1380p	-	YBL	<bminhd>	-	[Oh.
J06:1380q	-	AT	THE	the	[Ns.
J06:1380r	-	JJ	LIQUID	liquid	[Ns.
J06:1390a	-	NN1c	PHASE	phase	.Ns]
J06:1390b	-	JJ	PHOTOCHEMICAL	photochemical	.
J06:1390c	-	NN1n	REACTION	reaction	.Ns]
J06:1390d	-	YF	+.	-	.
J06:1390e	-	YBR	<eminhd>	-	.Oh]
J06:1390f	-	YD	<mdash>	-	[O.
J06:1390g	-	AT	The	the	[S[Ns:s.
J06:1390h	-	JJ	liquid	liquid	[Ns.
J06:1390i	-	NN1c	phase	phase	.Ns]
J06:1390j	-	JJ	photochemical	photochemical	.
J06:1400a	-	NN1n	exchange	exchange	.
J06:1400b	-	II	between	between	[P.
J06:1400c	-	NN1u	chlorine	chlorine	[N.
J06:1400d	-	CC	and	and	[Ns+.
J06:1400e	-	NN1n	carbon	carbon	.
J06:1400f	-	NN1u	tetrachloride	tetrachloride	.Ns+]N]P]Ns:s]
J06:1400g	-	VBDZ	was	be	[Vsb.Vsb]
J06:1400h	-	DAR	more	more	[Jh:e.
J06:1400i	-	JJ	reproducible	reproducible	.
J06:1410a	-	CSN	than	than	[P.
J06:1410b	-	AT	the	the	[Ns.
J06:1410c	-	JJ	thermal	thermal	.
J06:1410d	-	NN1n	exchange	exchange	.Ns]P]Jh:e]
J06:1410e	-	YC	+,	-	.
J06:1410f	-	CS	although	although	[Fa:c.
J06:1410g	-	RR	still	still	[R:t.R:t]
J06:1410h	-	JJ	erratic	erratic	[J:e.J:e]Fa:c]S]
J06:1410i	-	YF	+.	-	.
J06:1410j	-	AT	The	the	[S[Ns:s.
J06:1410k	-	NN1n	improvement	improvement	.Ns:s]
J06:1420a	-	VBDZ	was	be	[Vsb.Vsb]
J06:1420b	-	DAT	most	most	[J:e.
J06:1420c	-	JJ	noticeable	noticeable	.J:e]
J06:1420d	-	II	in	in	[P:r.
J06:1420e	-	AT	the	the	[Ns.
J06:1420f	-	JJR	greater	great	.
J06:1420g	-	NN1n	consistency	consistency	.
J06:1420h	-	II	among	among	[P.
J06:1420i	-	NN1n	reaction	reaction	[Np:197.
J06:1420j	-	NN2	cells	cell	.
J06:1420k	-	YG	-	-	[Tn[S197.S197]
J06:1430a	-	VVNv	prepared	prepare	[Vn.Vn]
J06:1430b	-	IIa	as	as	[P:h.
J06:1430c	-	AT1	a	a	[Ns.
J06:1430d	-	NNJ1c	group	group	.Ns]P:h]
J06:1430e	-	II	on	on	[P:p.
J06:1430f	-	AT	the	the	[Ns.
J06:1430g	-	DAy	same	same	.
J06:1430h	-	NN1c	manifold	manifold	.Ns]P:p]Tn]Np:197]P]Ns]P:r]S]
J06:1430i	-	YF	+.	-	.
J06:1430j	-	RGr	Rather	rather	[S[Np:S[J.
J06:1430k	-	JJ	large	large	.J]
J06:1430m	-	NN2	differences	difference	.
J06:1430n	-	YG	-	-	[199.199]Np:S]
J06:1430p	-	YG	-	-	[t201.t201]
J06:1430q	-	VBDR	were	be	[Vwp.
J06:1440a	-	RR	still	still	[R:G201.R:G201]
J06:1440b	-	VVNt	found	find	.Vwp]
J06:1440c	-	II	between	between	[P:G199.
J06:1440d	-	NN1n	reaction	reaction	[Np.
J06:1440e	-	NN2	cells	cell	.
J06:1440f	-	II	from	from	[P.
J06:1440g	-	JJ	different	different	[Np.
J06:1440h	-	NN1c	manifold	manifold	.
J06:1440i	-	NN2	fillings	filling	.Np]P]Np]P:G199]S]
J06:1440j	-	YF	+.	-	.
J06:1450a	-	DDi	Some	some	[S[Np:S.
J06:1450b	-	MCn	80	-	.
J06:1450c	-	NN1n	reaction	reaction	.
J06:1450d	-	NN2	tubes	tube	.
J06:1450e	-	II	from	from	[P.
J06:1450f	-	MCn	13	-	[Np.
J06:1450g	-	NN1c	manifold	manifold	.
J06:1450h	-	NN2	fillings	filling	.Np]P]Np:S]
J06:1450i	-	VBDR	were	be	[Vwp.
J06:1450j	-	VVNt	illuminated	illuminate	.Vwp]
J06:1450k	-	II	in	in	[P:p.
J06:1460a	-	AT	the	the	[Ns.
J06:1460b	-	NN1n	temperature	temperature	.
J06:1460c	-	NN1c	range	range	.
J06:1460d	-	II	from	from	[P.
J06:1460e	-	MCn	40	-	.P]
J06:1460f	-	IIt	to	to	[P.
J06:1460g	-	MCn	85	-	[Nu.
J06:1460h	-	NNU	+<deg>	-	.Nu]P]Ns]P:p]
J06:1460i	-	II	in	in	[P:h.
J06:1460j	-	AT1	a	a	[Ns.
J06:1460k	-	JJR	further	far	.
J06:1460m	-	NN1c	endeavor	endeavour	.
J06:1460n	-	TO	to	to	[Ti[Vi.
J06:1460p	-	VV0v	determine	determine	.Vi]
J06:1470a	-	AT	the	the	[Ns:o.
J06:1470b	-	NN1n	cause	cause	.
J06:1470c	-	IO	of	of	[Po.
J06:1470d	-	AT	the	the	[Ns.
J06:1470e	-	NN1u	irreproducibility	irreproducibility	.Ns]Po]Ns:o]
J06:1470f	-	CC	and	and	[Ti+.
J06:1470g	-	TO	to	to	[Vi.
J06:1470h	-	VV0v	obtain	obtain	.Vi]
J06:1470i	-	NN1u	information	information	[Ns:o.
J06:1470j	-	II	on	on	[P.
J06:1480a	-	AT	the	the	[N.
J06:1480b	-	NN1c	activation	activation	.
J06:1480c	-	NN1n	energy	energy	.
J06:1480d	-	CC	and	and	[Ns+.
J06:1480e	-	AT	the	the	.
J06:1480f	-	NN1n	effect	effect	.
J06:1480g	-	IO	of	of	[Po.
J06:1480h	-	NN1n	light	light	[Ns.
J06:1480i	-	NN1n	intensity	intensity	.Ns]Po]Ns+]N]P]Ns:o]Ti+]Ti]Ns]P:h]S]
J06:1480j	-	YF	+.	-	.
J06:1480k	-	II	In	in	[S[P:r.
J06:1480m	-	DBa	all	all	[Np.
J06:1480n	-	NN2	cases	case	.Np]P:r]
J06:1490a	-	EX	there	there	.
J06:1490b	-	VBDZ	was	be	[Vsb.Vsb]
J06:1490c	-	RR	readily	readily	[Ns:s[J.
J06:1490d	-	JJ	measurable	measurable	.J]
J06:1490e	-	NN1n	exchange	exchange	.Ns:s]
J06:1490f	-	ICSt	after	after	[P:t.
J06:1490g	-	RGa	as	as	[Ds.
J06:1490h	-	DA1	little	little	.
J06:1490i	-	CSA	as	as	[P.
J06:1490j	-	MC1	one	one	[Ns.
J06:1490k	-	NNT1c	hour	hour	.Ns]P]
J06:1490m	-	IO	of	of	[Po.
J06:1500a	-	NN1n	illumination	illumination	.Po]Ds]P:t]S]
J06:1500b	-	YF	+.	-	.
J06:1500c	-	IIb	By	by	[S[Pb:h.
J06:1500d	-	VVGv	comparing	compare	[Tg[Vg.Vg]
J06:1500e	-	NN1n	reaction	reaction	[Np:o203.
J06:1500f	-	NN2	cells	cell	.
J06:1500g	-	YG	-	-	[Tn[S203.S203]
J06:1500h	-	VVNv	sealed	seal	[Vn.Vn]
J06:1500i	-	II	from	from	[P:q.
J06:1500j	-	AT	the	the	[Ns.
J06:1500k	-	DAy	same	same	.
J06:1500m	-	NN1c	manifold	manifold	.Ns]P:q]Tn]Np:o203]Tg]Pb:h]
J06:1510a	-	NN1n	temperature	temperature	[Ns:s205.
J06:1510b	-	NN1c	dependency	dependency	.
J06:1510c	-	YG	-	-	[Tg[s205.s205]
J06:1510d	-	VVGi	corresponding	correspond	[Vg.Vg]
J06:1510e	-	IIt	to	to	[P:u.
J06:1510f	-	NN1c	activation	activation	[Np:207.
J06:1510g	-	NN2	energies	energy	.
J06:1510h	-	YG	-	-	[Tg[s207.s207]
J06:1510i	-	VVGv	ranging	range	[Vg.Vg]
J06:1520a	-	II	from	from	[P:q.
J06:1520b	-	MCn	11	-	.P:q]
J06:1520c	-	IIt	to	to	[P:q.
J06:1520d	-	MCn	18	-	[N.
J06:1520e	-	FO	<formul>	-	.N]P:q]Tg]Np:207]P:u]Tg]Ns:s205]
J06:1520f	-	VBDZ	was	be	[Vsp.
J06:1520g	-	VVNv	observed	observe	.Vsp]
J06:1520h	-	CS	while	while	[Fa:c.
J06:1520i	-	NN1u	dependence	dependence	[Ns:S209.
J06:1520j	-	II	on	on	[P.
J06:1520k	-	AT	the	the	[Ns.
J06:1520m	-	MDo	first	first	.
J06:1520n	-	NN1n	power	power	.
J06:1520p	-	IO	of	of	[Po.
J06:1530a	-	AT	the	the	[Ns.
J06:1530b	-	NN1n	light	light	.
J06:1530c	-	NN1n	intensity	intensity	.Ns]Po]Ns]P]Ns:S209]
J06:1530d	-	VVDi	seemed	seem	[Vd.Vd]
J06:1530e	-	YG	-	-	[Ti:s[S209.S209]
J06:1530f	-	TO	to	to	[Vip.
J06:1530g	-	VB0	be	be	.
J06:1530h	-	VVNt	indicated	indicate	.Vip]
J06:1530i	-	II	in	in	[P:m.
J06:1530j	-	DAT	most	most	[Np.
J06:1530k	-	NN2	cases	case	.Np]P:m]Ti:s]Fa:c]S]O]
J06:1530m	-	YB	<minbrk>	-	[Oh.Oh]
J06:1530n	-	PPH1	It	it	[O[S[Ni:S.Ni:S]
J06:1540a	-	VBDZ	was	be	[Vsb.Vsb]
J06:1540b	-	JJ	possible	possible	[J:e.J:e]
J06:1540c	-	TO	to	to	[Ti:s[Vi.
J06:1540d	-	VV0v	make	make	.Vi]
J06:1540e	-	NN2	estimates	estimate	[Np:o.
J06:1540f	-	IO	of	of	[Po.
J06:1540g	-	AT	the	the	[Ns.
J06:1540h	-	NN1c	quantum	quantum	.
J06:1540i	-	NN1n	yield	yield	.Ns]Po]Np:o]
J06:1540j	-	IIb	by	by	[Pb:h.
J06:1540k	-	VVGv	observing	observe	[Tg[Tg&[Vg.Vg]
J06:1540m	-	AT	the	the	[Ns:o.
J06:1540n	-	NN1u	extent	extent	.
J06:1550a	-	IO	of	of	[Po.
J06:1550b	-	NN1n	reduction	reduction	[Ns.
J06:1550c	-	IO	of	of	[Po.
J06:1550d	-	AT1	a	a	[Ns:211.
J06:1550e	-	NN1n	uranyl	uranyl	[Ns.
J06:1550f	-	NN1u	oxalate	oxalate	.Ns]
J06:1550g	-	NN1c	actinometer	actinometer	.
J06:1550h	-	NN1n	solution	solution	.
J06:1550i	-	YG	-	-	[Tn[S211.S211]
J06:1550j	-	VVNt	illuminated	illuminate	[Vn.Vn]
J06:1560a	-	IF	for	for	[P:t.
J06:1560b	-	AT1	a	a	[Ns.
J06:1560c	-	VVNv	known	know	[Tn[Vn.Vn]Tn]
J06:1560d	-	NNT1c	time	time	.Ns]P:t]
J06:1560e	-	II	in	in	[P:p.
J06:1560f	-	AT1	a	a	[Ns.
J06:1560g	-	JJ	typical	typical	.
J06:1560h	-	NN1n	reaction	reaction	.
J06:1560i	-	NN1c	cell	cell	.Ns]P:p]Tn]Ns:211]Po]Ns]Po]Ns:o]
J06:1560j	-	CC	and	and	[Tg+.
J06:1560k	-	VVGv	making	make	[Vg.Vg]
J06:1560m	-	JJ	appropriate	appropriate	[Np:o213.
J06:1560n	-	NN2	conversions	conversion	.
J06:1560p	-	YG	-	-	[Tn[S213.S213]
J06:1570a	-	VVNt	based	base	[Vn.Vn]
J06:1570b	-	II	on	on	[P:u.
J06:1570c	-	AT	the	the	[Np.
J06:1570d	-	NN2	differences	difference	.
J06:1570e	-	II	in	in	[P.
J06:1570f	-	AT	the	the	[Np.
J06:1570g	-	NN1u	absorption	absorption	.
J06:1570h	-	NN2	spectra	spectrum	.
J06:1570i	-	IO	of	of	[Po.
J06:1570j	-	NN1n	uranyl	uranyl	[Ns.
J06:1580a	-	NN1u	oxalate	oxalate	.Ns]
J06:1580b	-	CC	and	and	[Po+.
J06:1580c	-	IO	of	of	.
J06:1580d	-	NN1u	chlorine	chlorine	.Po+]Po]Np]P]Np]P:u]Tn]Np:o213]Tg+]Tg&]
J06:1580e	-	YC	+,	-	.
J06:1580f	-	CC	and	and	[Tg+.
J06:1580g	-	VVGt	considering	consider	[Vg.Vg]
J06:1580h	-	AT	the	the	[Ns:o.
J06:1580i	-	JJ	spectral	spectral	.
J06:1580j	-	NN1n	distribution	distribution	.
J06:1580k	-	IO	of	of	[Po.
J06:1590a	-	AT	the	the	[Ns.
J06:1590b	-	NN1n	light	light	.
J06:1590c	-	NN1c	source	source	.Ns]Po]Ns:o]Tg+]Tg]Pb:h]Ti:s]S]
J06:1590d	-	YF	+.	-	.
J06:1590e	-	DD2i	These	these	[S[Np:s.
J06:1590f	-	NN2	estimates	estimate	.Np:s]
J06:1590g	-	VVDt	indicated	indicate	[Vd.Vd]
J06:1590h	-	CST	that	that	[Fn:o.
J06:1590i	-	AT	the	the	[Ns:s.
J06:1590j	-	NN1c	quantum	quantum	.
J06:1590k	-	NN1n	yield	yield	.
J06:1600a	-	IF	for	for	[P.
J06:1600b	-	AT	the	the	[Ns.
J06:1600c	-	NN1n	exchange	exchange	.
J06:1600d	-	IO	of	of	[Po.
J06:1600e	-	NN1u	chlorine	chlorine	.Po]
J06:1600f	-	IW	with	with	[P.
J06:1600g	-	JJ	liquid	liquid	[Ns.
J06:1600h	-	NN1n	carbon	carbon	.
J06:1600i	-	NN1u	tetrachloride	tetrachloride	.Ns]P]
J06:1600j	-	II	at	at	[P.
J06:1600k	-	MCn	65	-	[Nu.
J06:1600m	-	NNU	+<deg>	-	.Nu]P]Ns]P]Ns:s]
J06:1610a	-	VBZ	is	be	[Vzb.Vzb]
J06:1610b	-	IO	of	of	[Po:e.
J06:1610c	-	AT	the	the	[Ns.
J06:1610d	-	NN1n	order	order	.
J06:1610e	-	IO	of	of	[Po.
J06:1610f	-	NN1u	magnitude	magnitude	.Po]
J06:1610g	-	IO	of	of	[Po.
J06:1610h	-	NN1n	unity	unity	.Po]Ns]Po:e]Fn:o]S]
J06:1610i	-	YF	+.	-	.O]
J06:1610j	-	YB	<minbrk>	-	[Oh.Oh]
J06:1610k	-	CSn	When	when	[O[S[Fa:t[Rq:t.Rq:t]
J06:1610m	-	JJ	typical	typical	[Np:S215.
J06:1610n	-	NN1n	reaction	reaction	.
J06:1620a	-	NN2	cells	cell	.
J06:1620b	-	IIt	to	to	[Fr[Pq:q.
J06:1620c	-	DDQr	which	which	[Dq:215.Dq:215]Pq:q]
J06:1620d	-	MCd	0.3	-	[M:S.
J06:1620e	-	IO	of	of	[Po.
J06:1620f	-	AT1	an	an	[Ns.
J06:1620g	-	NN1n	atmosphere	atmosphere	.Ns]Po]
J06:1620h	-	IO	of	of	[Po.
J06:1620i	-	NN1u	oxygen	oxygen	.Po]M:S]
J06:1620j	-	VHD	had	have	[Vdfp.
J06:1620k	-	VBN	been	be	.
J06:1620m	-	VVNv	added	add	.Vdfp]Fr]Np:S215]
J06:1620n	-	VBDR	were	be	[Vwp.
J06:1620p	-	VVNt	illuminated	illuminate	.Vwp]Fa:t]
J06:1620q	-	YC	+,	-	.
J06:1630a	-	NN1u	chlorine	chlorine	[N:S[NN1u&.
J06:1630b	-	CC	and	and	[NN1u+.
J06:1630c	-	NN1u	phosgene	phosgene	.NN1u+]NN1u&]N:S]
J06:1630d	-	VBDR	were	be	[Vwp.
J06:1630e	-	VVNv	produced	produce	.Vwp]S]
J06:1630f	-	YF	+.	-	.
J06:1630g	-	NN1n	Exchange	exchange	[S[Ns:S.Ns:S]
J06:1630h	-	YG	-	-	[m217.m217]
J06:1630i	-	VBDZ	was	be	[Vsp.
J06:1630j	-	RR	also	also	[R:G217.R:G217]
J06:1630k	-	VVNv	observed	observe	.Vsp]
J06:1640a	-	II	in	in	[P:p.
J06:1640b	-	DD2i	these	these	[Np:219.
J06:1640c	-	NN2	cells	cell	.
J06:1640d	-	YC	+,	-	.
J06:1640e	-	DDQr	which	which	[Fr[Dq:s219.Dq:s219]
J06:1640f	-	VHD	had	have	[Vd.Vd]
J06:1640g	-	NN1u	chlorine	chlorine	[Ns:o.Ns:o]
J06:1640h	-	JJ	present	present	[J:e.J:e]
J06:1640i	-	II	at	at	[P:p.
J06:1640j	-	FO	<formul>	-	.P:p]Fr]Np:219]P:p]S]
J06:1640k	-	YF	+.	-	.O]
J06:1640m	-	YBL	<bminhd>	-	[Oh.
J06:1640n	-	AT	THE	the	[Ns.
J06:1640p	-	JJ	PHOTOCHEMICAL	photochemical	.
J06:1650a	-	NN1n	EXCHANGE	exchange	.
J06:1650b	-	II	IN	in	[P.
J06:1650c	-	AT	THE	the	[Ns.
J06:1650d	-	NN1n	GAS	gas	.
J06:1650e	-	NN1c	PHASE	phase	.Ns]P]Ns]
J06:1650f	-	YF	+.	-	.
J06:1650g	-	YBR	<eminhd>	-	.Oh]
J06:1650h	-	YD	<mdash>	-	[O.
J06:1650i	-	CS	Although	although	[S[Fa:c.
J06:1650j	-	EX	there	there	.
J06:1650k	-	VBDZ	was	be	[Vsb.Vsb]
J06:1650m	-	DDi	some	some	[Ns:s221.
J06:1650n	-	NN1n	variation	variation	.
J06:1660a	-	II	in	in	[P.
J06:1660b	-	NN2	results	result	.P]
J06:1660c	-	DDQr	which	which	[Fr[Dq:S221.Dq:S221]
J06:1660d	-	VMo	must	must	[Vcp.
J06:1660e	-	VB0	be	be	.
J06:1660f	-	VVNt	attributed	attribute	.Vcp]
J06:1660g	-	LEe	either	either	[P:u.
J06:1660h	-	IIt	to	to	.
J06:1660i	-	NN1n	trace	trace	[Np.
J06:1660j	-	NN2	impurities	impurity	.Np]
J06:1660k	-	CCr	or	or	[P+.
J06:1670a	-	IIt	to	to	.
J06:1670b	-	NN1n	variation	variation	[Ns.
J06:1670c	-	II	in	in	[P.
J06:1670d	-	NN1c	wall	wall	[Np.
J06:1670e	-	NN2	effects	effect	.Np]P]Ns]P+]P:u]Fr]Ns:s221]Fa:c]
J06:1670f	-	YC	+,	-	.
J06:1670g	-	AT	the	the	[Ns:s.
J06:1670h	-	JJ	photochemical	photochemical	.
J06:1670i	-	NN1n	exchange	exchange	.
J06:1670j	-	II	in	in	[P.
J06:1670k	-	AT	the	the	[Ns.
J06:1670m	-	NN1n	gas	gas	.
J06:1670n	-	NN1c	phase	phase	.Ns]P]Ns:s]
J06:1680a	-	VBDZ	was	be	[Vsb.Vsb]
J06:1680b	-	RR	sufficiently	sufficiently	[Jh:e.
J06:1680c	-	JJ	reproducible	reproducible	.
J06:1680d	-	RRz	so	so	[R.
J06:1680e	-	CST	that	that	[Fc.
J06:1680f	-	PPH1	it	it	[Ni:S.Ni:S]
J06:1680g	-	VVDi	seemed	seem	[Vd.Vd]
J06:1680h	-	JJ	meaningful	meaningful	[J:e.J:e]
J06:1680i	-	TO	to	to	[Ti:s[Vi.
J06:1680j	-	VV0v	compare	compare	.Vi]
J06:1690a	-	AT	the	the	[Np:o.
J06:1690b	-	NN1n	reaction	reaction	.
J06:1690c	-	NN2	rates	rate	.
J06:1690d	-	II	in	in	[P.
J06:1690e	-	JJ	different	different	[N.
J06:1690f	-	NNc	series	series	.
J06:1690g	-	IO	of	of	[Po.
J06:1690h	-	NN1n	reaction	reaction	[Np.
J06:1690i	-	NN2	tubes	tube	.Np]Po]N]P]Np:o]
J06:1690j	-	IF	for	for	[P:c.
J06:1690k	-	AT	the	the	[Ns.
J06:1690m	-	NN1n	purpose	purpose	.
J06:1700a	-	IO	of	of	[Po.
J06:1700b	-	VVGv	obtaining	obtain	[Tg[Vg.Vg]
J06:1700c	-	NN1u	information	information	[Ns:o.
J06:1700d	-	II	on	on	[P.
J06:1700e	-	AT	the	the	[Ns.
J06:1700f	-	NN1n	effect	effect	.
J06:1700g	-	IO	of	of	[Po.
J06:1700h	-	NN1u	chlorine	chlorine	[Ns.
J06:1700i	-	NN1n	concentration	concentration	.Ns]
J06:1710a	-	CC	and	and	[Po+.
J06:1710b	-	IO	of	of	.
J06:1710c	-	NN1n	carbon	carbon	[Ns[Ns.
J06:1710d	-	NN1u	tetrachloride	tetrachloride	.Ns]
J06:1710e	-	NN1n	concentration	concentration	.Ns]Po+]Po]
J06:1710f	-	II	on	on	[P.
J06:1710g	-	AT	the	the	[Ns.
J06:1710h	-	NN1n	reaction	reaction	.
J06:1710i	-	NN1c	rate	rate	.Ns]P]Ns]P]Ns:o]Tg]Po]Ns]P:c]Ti:s]Fc]R]Jh:e]S]
J06:1710j	-	YF	+.	-	.
J06:1710k	-	NNu	Data	data	[S[N:S.
J06:1720a	-	II	on	on	[P.
J06:1720b	-	DAz	such	such	[Np.
J06:1720c	-	NN2	comparisons	comparison	.Np]P]
J06:1720d	-	II21	together	together	[P[II=.
J06:1720e	-	II22	with	with	.II=]
J06:1720f	-	NNu	data	data	[N.
J06:1720g	-	II	on	on	[P.
J06:1720h	-	AT	the	the	[Ns.
J06:1720i	-	NN1n	effect	effect	.
J06:1720j	-	IO	of	of	[Po.
J06:1720k	-	NN1n	light	light	[Ns.
J06:1720m	-	NN1n	intensity	intensity	.Ns]Po]Ns]P]N]P]N:S]
J06:1730a	-	VBR	are	be	[Vap.
J06:1730b	-	VVNv	given	give	.Vap]
J06:1730c	-	II	in	in	[P:p.
J06:1730d	-	NN1c	Table	table	[Nns.
J06:1730e	-	MCr	I	-	.Nns]P:p]S]
J06:1730f	-	YF	+.	-	.O]
J06:1730g	-	YB	<minbrk>	-	[Oh.Oh]
J06:1730h	-	II	In	in	[O[S[P:p.
J06:1730i	-	NNc	series	series	[Nn.
J06:1730j	-	MCr	I	-	.Nn]P:p]
J06:1730k	-	AT	the	the	[Ns:S.
J06:1730m	-	JJ	relative	relative	.
J06:1730n	-	NN1n	light	light	.
J06:1740a	-	NN1n	intensity	intensity	.Ns:S]
J06:1740b	-	VBDZ	was	be	[Vsp.
J06:1740c	-	VVNv	varied	vary	.Vsp]
J06:1740d	-	IIb	by	by	[Pb:h.
J06:1740e	-	VVGv	varying	vary	[Tg[Vg.Vg]
J06:1740f	-	AT	the	the	[Ns:o.
J06:1740g	-	NN1n	distance	distance	.
J06:1740h	-	IO	of	of	[Po.
J06:1740i	-	AT	the	the	[Ns.
J06:1740j	-	NN1c	lamp	lamp	.Ns]Po]
J06:1740k	-	II	from	from	[P.
J06:1740m	-	AT	the	the	[Ns.
J06:1750a	-	NN1n	reaction	reaction	.
J06:1750b	-	NN1c	cell	cell	.Ns]P]Ns:o]
J06:1750c	-	II	over	over	[P:p.
J06:1750d	-	AT	the	the	[Ns.
J06:1750e	-	NN1c	range	range	.
J06:1750f	-	II	from	from	[P.
J06:1750g	-	MCd	14.7	-	.P]
J06:1750h	-	IIt	to	to	[P.
J06:1750i	-	MCd	29.2	-	[Nu.
J06:1750j	A	NNU	cm	-	.Nu]P]Ns]P:p]Tg]Pb:h]S]
J06:1750k	-	YF	+.	-	.
J06:1750m	-	AT	The	the	[S[Ns:s.
J06:1750n	-	MDt	last	last	.
J06:1750p	-	NN1c	column	column	.Ns:s]
J06:1760a	-	VVZv	shows	show	[Vz.Vz]
J06:1760b	-	AT	the	the	[Ns:o223.
J06:1760c	-	NN1c	rate	rate	.
J06:1760d	-	IO	of	of	[Po.
J06:1760e	-	NN1n	exchange	exchange	.Po]
J06:1760f	-	CST	that	that	[Fr.
J06:1760g	-	YG	-	-	[S223.S223]
J06:1760h	-	VMd	would	will	[Vdcfp.
J06:1760i	-	VH0	have	have	.
J06:1760j	-	VBN	been	be	.
J06:1760k	-	VVNv	observed	observe	.Vdcfp]
J06:1760m	-	II	at	at	[P:p.
J06:1760n	-	AT1	a	a	[Ns.
J06:1760p	-	JJ	relative	relative	.
J06:1770a	-	NN1n	intensity	intensity	.
J06:1770b	-	IO	of	of	[Po.
J06:1770c	-	MCn	4	-	.Po]
J06:1770d	-	YPL	(	-	.
J06:1770e	-	MCd	+14.7	-	[Ns@[Nu.
J06:1770f	A	NNU	cm.	-	.Nu]
J06:1770g	-	NN1n	distance	distance	.Ns@]
J06:1770h	-	YPR	+)	-	.Ns]P:p]Fr]
J06:1770i	-	YG	-	-	[Tn[S223.S223]
J06:1770j	-	VVNv	calculated	calculate	[Vn.Vn]
J06:1770k	-	II	on	on	[P:h.
J06:1770m	-	AT	the	the	[Np.
J06:1770n	-	NN2	assumptions	assumption	.
J06:1770p	-	CST	that	that	[Fn.
J06:1780a	-	AT	the	the	[Ns:s.
J06:1780b	-	NN1c	incident	incident	.
J06:1780c	-	NN1n	light	light	.
J06:1780d	-	NN1n	intensity	intensity	.Ns:s]
J06:1780e	-	VBZ	is	be	[Vzb.Vzb]
J06:1780f	-	RR	inversely	inversely	[Jh:e.
J06:1780g	-	JJ	proportional	proportional	.
J06:1780h	-	IIt	to	to	[P.
J06:1780i	-	AT	the	the	[Ns.
J06:1780j	-	NNL1c	square	square	.
J06:1790a	-	IO	of	of	[Po.
J06:1790b	-	AT	the	the	[Ns.
J06:1790c	-	NN1n	distance	distance	.
J06:1790d	-	IO	of	of	[Po.
J06:1790e	-	AT	the	the	[Ns.
J06:1790f	-	NN1c	lamp	lamp	.Ns]Po]
J06:1790g	-	II	from	from	[P.
J06:1790h	-	AT	the	the	[Ns.
J06:1790i	-	NN1c	cell	cell	.Ns]P]Ns]Po]Ns]P]Jh:e]
J06:1790j	-	CC	and	and	[Fn+.
J06:1790k	-	CST	that	that	.
J06:1790m	-	AT	the	the	[Ns:s.
J06:1790n	-	NN1c	rate	rate	.Ns:s]
J06:1790p	-	VBZ	is	be	[Vzb.Vzb]
J06:1790q	-	RR	directly	directly	[Jh:e.
J06:1800a	-	JJ	proportional	proportional	.
J06:1800b	-	IIt	to	to	[P.
J06:1800c	-	AT	the	the	[Ns.
J06:1800d	-	NN1c	incident	incident	.
J06:1800e	-	NN1n	light	light	.
J06:1800f	-	NN1n	intensity	intensity	.Ns]P]Jh:e]Fn+]Fn]Np]P:h]Tn]Ns:o223]S]
J06:1800g	-	YF	+.	-	.
J06:1800h	-	JJ	Direct	direct	[S[Ns:S.
J06:1800i	-	NN1u	proportionality	proportionality	.
J06:1810a	-	IO	of	of	[Po.
J06:1810b	-	AT	the	the	[Ns.
J06:1810c	-	NN1c	rate	rate	.Ns]Po]
J06:1810d	-	IIt	to	to	[P.
J06:1810e	-	AT	the	the	[Ns.
J06:1810f	-	NN1c	incident	incident	.
J06:1810g	-	NN1n	intensity	intensity	.Ns]P]Ns:S]
J06:1810h	-	YG	-	-	[m225.m225]
J06:1810i	-	VHZ	has	have	[Vzfp.
J06:1810j	-	RR	also	also	[R:G225.R:G225]
J06:1810k	-	VBN	been	be	.
J06:1810m	-	VVNt	assumed	assume	.Vzfp]
J06:1810n	-	II	in	in	[P:t.
J06:1810p	-	VVGv	obtaining	obtain	[Tg[Vg.Vg]
J06:1820a	-	AT	the	the	[Ns:o.
J06:1820b	-	NN1n	value	value	.
J06:1820c	-	II	in	in	[P.
J06:1820d	-	AT	the	the	[Ns.
J06:1820e	-	MDt	last	last	.
J06:1820f	-	NN1c	column	column	.Ns]P]
J06:1820g	-	IF	for	for	[P.
J06:1820h	-	AT	the	the	[Ns:227.
J06:1820i	-	MD	fourth	fourth	.
J06:1820j	-	NN1c	sample	sample	.
J06:1820k	-	IO	of	of	[Po.
J06:1820m	-	NNc	series	series	[Nn.
J06:1820n	-	MCr	II	-	.Nn]Po]
J06:1830a	-	RRQr	where	where	[Fr[Rq:p227.Rq:p227]
J06:1830b	-	AT	the	the	[Ns:S.
J06:1830c	-	NN1n	light	light	.
J06:1830d	-	NN1n	intensity	intensity	.Ns:S]
J06:1830e	-	VBDZ	was	be	[Vsp.
J06:1830f	-	VVNv	reduced	reduce	.Vsp]
J06:1830g	-	IIb	by	by	[Pb:h.
J06:1830h	-	NN1n	use	use	[Ns.
J06:1830i	-	IO	of	of	[Po.
J06:1830j	-	AT1	a	a	[Ns.
J06:1830k	-	NN1c	screen	screen	.Ns]Po]Ns]Pb:h]Fr]Ns:227]P]Ns:o]Tg]P:t]S]
J06:1830m	-	YF	+.	-	.O]
